Thermodynamic study on solar thermochemical fuel production with oxygen permeation membrane reactors

CORC > 工程热物理研究所 > 中国科学院工程热物理研究所 > 中国科学院工程热物理所（论文库） > 期刊论文（SCI）

	Thermodynamic study on solar thermochemical fuel production with oxygen permeation membrane reactors
	Wang, Hongsheng 1,2; Hao, Yong 1; Kong, Hui 1,2
刊名	INTERNATIONAL JOURNAL OF ENERGY RESEARCH
	2015-10-25
卷号	39 期号:13 页码:1790-1799
关键词	solar thermochemistry isothermal water splitting methane syngas oxygen permeation membrane
英文摘要	Thermodynamic analysis is performed on a conceptual oxygen permeation membrane reactor driven by concentrated solar energy (heat) for isothermal H2O splitting for the purpose of solar fuel derivation. By way of a plug-flow reactor model, kinetic and thermodynamic factors responsible for conversion rate, reactor dimension, and solar-to-fuel efficiency are analyzed for the case of pump-assisted and methane-assisted scenarios. The pump-assisted case achieves the same solar-to-fuel efficiency (2.9% at 1500 degrees C) as isothermal solar thermochemical cycling, while the methane-assisted case attains much higher efficiencies at much lower temperatures, whose net solar-to-fuel efficiency reaches 63% at around 900 degrees C. The theoretical framework developed in this study can be applied to the solar thermochemical splitting of other gases such as CO2 and can be further extended to the co-splitting of H2O and CO2 for syngas production driven by solar energy only (i.e., without the participation of hydrocarbon fuels). Copyright (c) 2015 John Wiley & Sons, Ltd.
WOS标题词	Science & Technology ; Technology
类目[WOS]	Energy & Fuels ; Nuclear Science & Technology
研究领域[WOS]	Energy & Fuels ; Nuclear Science & Technology
关键词[WOS]	HYDROGEN ; WATER ; METHANE
收录类别	SCI
语种	英语
WOS记录号	WOS:000362581000007
公开日期	2015-12-22
内容类型	期刊论文
源URL	[http://ir.etp.ac.cn/handle/311046/101566]
专题	工程热物理研究所_中国科学院工程热物理所（论文库）_期刊论文（SCI）
作者单位	1.Chinese Acad Sci, Inst Engn Thermophys, Beijing 100190, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
推荐引用方式 GB/T 7714	Wang, Hongsheng,Hao, Yong,Kong, Hui. Thermodynamic study on solar thermochemical fuel production with oxygen permeation membrane reactors[J]. INTERNATIONAL JOURNAL OF ENERGY RESEARCH,2015,39(13):1790-1799.
APA	Wang, Hongsheng,Hao, Yong,&Kong, Hui.(2015).Thermodynamic study on solar thermochemical fuel production with oxygen permeation membrane reactors.INTERNATIONAL JOURNAL OF ENERGY RESEARCH,39(13),1790-1799.
MLA	Wang, Hongsheng,et al."Thermodynamic study on solar thermochemical fuel production with oxygen permeation membrane reactors".INTERNATIONAL JOURNAL OF ENERGY RESEARCH 39.13(2015):1790-1799.