Size-selective self-assembly of magnetic Mn nanoclusters on Si(111) | |
Niu, CY ; Wang, JT ; Wang, EG ; Chen, CF | |
刊名 | JOURNAL OF CHEMICAL PHYSICS |
2013 | |
卷号 | 138期号:16 |
ISSN号 | 0021-9606 |
通讯作者 | Niu, CY (reprint author), Chinese Acad Sci, Inst Phys, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. |
中文摘要 | We show by first-principles calculations two types of magnetic magic Mn clusters on the Si(111)-(7x7) surface. The first is a small triangular Mn-7 cluster stabilized by the solid-centered Mn-Si-3 bonds on the top layer, and the second is a large hexagonal Mn-13 cluster favored by the confining potential wells of the faulted half unit cells on the Si(111) surface. These two structural models are distinct from that of the planar group-III clusters on Si(111) and produce simulated scanning tunneling microscopy images in reasonable agreement with recent experimental observations. These results offer key insights for understanding the complex energetic landscape on the Si(111)-(7x7) surface, which is critical to precisely controlled growth of Mn nanocluster arrays with specific size, magnetic moment, and good uniformity. (C) 2013 AIP Publishing LLC. |
资助信息 | National Natural Science Foundation of China (NNSFC) [10974230, 11274356]; DOE [DE-FC52-06NA27684] |
语种 | 英语 |
公开日期 | 2014-01-17 |
内容类型 | 期刊论文 |
源URL | [http://ir.iphy.ac.cn/handle/311004/57447] |
专题 | 物理研究所_物理所公开发表论文_物理所公开发表论文_期刊论文 |
推荐引用方式 GB/T 7714 | Niu, CY,Wang, JT,Wang, EG,et al. Size-selective self-assembly of magnetic Mn nanoclusters on Si(111)[J]. JOURNAL OF CHEMICAL PHYSICS,2013,138(16). |
APA | Niu, CY,Wang, JT,Wang, EG,&Chen, CF.(2013).Size-selective self-assembly of magnetic Mn nanoclusters on Si(111).JOURNAL OF CHEMICAL PHYSICS,138(16). |
MLA | Niu, CY,et al."Size-selective self-assembly of magnetic Mn nanoclusters on Si(111)".JOURNAL OF CHEMICAL PHYSICS 138.16(2013). |
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