S vacancy in MoS<sub>2</sub> nanosheets induces H<sub>2</sub>O cleavage: a new era for 2D nanozyme

doi:10.1007/s11164-023-05135-y

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	S vacancy in MoS₂ nanosheets induces H₂O cleavage: a new era for 2D nanozyme
	Wang, Jin 4,5,6; Ren, Wenyu 4,6; Wang, Yi 4,5,6; Zhang, Dun 4,5,6; Wang, Yu 3; Ju, Peng 2; Dou, Kunpeng 1
刊名	RESEARCH ON CHEMICAL INTERMEDIATES
	2023-09-21
卷号	49 期号:12 页码:10
关键词	MoS2 Nanozyme Peroxidase-like activity S vacancy DFT calculations
ISSN号	0922-6168
DOI	10.1007/s11164-023-05135-y
通讯作者	Wang, Yi(wangyi@qdio.ac.cn)
英文摘要	Nanozyme is a promising approach in treating pollution in drinking water sources. 2D MoS2 nanosheets, with abundant active sites and Lewis acid sites, exhibit outstanding peroxidase-like activity. Verified by density functional calculation, S vacancies in 2D MoS2 nanosheets can cleavage H2O to yield H+ and .OH. The spontaneous generation of acid environment and oxygen free radicals enables 2D MoS2 nanosheets to be effectively exploited in the depuration of polluted water, creating a new era for multifunctional nanozymes.
资助项目	Natural Science Foundation of China[42176047] ; Second Batch of Postdoctoral Funding in Qingdao in 2022 ; 2022 Special Research Assistant Program of the Chinese Academy of Science ; 73rd batch of general support from China Postdoctoral Science Foundation
WOS关键词	PEROXIDASE-LIKE ACTIVITY ; REDUCTION ; ENZYMES
WOS研究方向	Chemistry
语种	英语
出版者	SPRINGER
WOS记录号	WOS:001071123100004
内容类型	期刊论文
源URL	[http://ir.qdio.ac.cn/handle/337002/181534]
专题	海洋研究所_海洋腐蚀与防护研究发展中心
通讯作者	Wang, Yi
作者单位	1.Ocean Univ China, Coll Informat Sci & Engn, Qingdao 266100, Peoples R China 2.Minist Nat Resources, Inst Oceanog 1, Marine Bioresource & Environm Res Ctr, Key Lab Marine Ecoenvironm Sci & Technol, Qingdao 266061, Peoples R China 3.Soochow Univ, Coll Pharmaceut Sci, Suzhou 215123, Peoples R China 4.Pilot Natl Lab Marine Sci & Technol, Open Studio Marine Corros & Protect, Qingdao 266237, Peoples R China 5.Univ Chinese Acad Sci, Beijing 100039, Peoples R China 6.Chinese Acad Sci, Inst Oceanol, CAS Key Lab Marine Environm Corros & Biofouling, Qingdao 266071, Peoples R China
推荐引用方式 GB/T 7714	Wang, Jin,Ren, Wenyu,Wang, Yi,et al. S vacancy in MoS₂ nanosheets induces H₂O cleavage: a new era for 2D nanozyme[J]. RESEARCH ON CHEMICAL INTERMEDIATES,2023,49(12):10.
APA	Wang, Jin.,Ren, Wenyu.,Wang, Yi.,Zhang, Dun.,Wang, Yu.,...&Dou, Kunpeng.(2023).S vacancy in MoS₂ nanosheets induces H₂O cleavage: a new era for 2D nanozyme.RESEARCH ON CHEMICAL INTERMEDIATES,49(12),10.
MLA	Wang, Jin,et al."S vacancy in MoS₂ nanosheets induces H₂O cleavage: a new era for 2D nanozyme".RESEARCH ON CHEMICAL INTERMEDIATES 49.12(2023):10.