Revealing the Modulation Effects on the Electronic Band Structures and Exciton Properties by Stacking Graphene/h-BN/MoS2Schottky Heterostructures
X. Zhu; J. He; W. Liu; Y. Zheng; C. Sheng; Y. Luo; S. Li; R. Zhang and J. Chu
2022
ISSN号19448244
DOI10.1021/acsami.2c20100
英文摘要Stacking two dimensional tunneling heterostructures has always been an important strategy to improve the optoelectronic device performance. However, there are still many disputes about the blocking ability of monolayer (1L-) h-BN on the interlayer coupling. Graphene/h-BN/MoS2 optoelectronic devices have been reported for superior device results. In this study, starting with graphene/h-BN/MoS2 heterostructures, we report experimental evidence of 1L-h-BN barrier layer modulation effects about the electronic band structures and exciton properties. We find that 1L-h-BN insertion only partially blocks the interlayer carrier transfer. In the meantime, the 1L-h-BN barrier layer weakens the interlayer coupling effect, by decreasing the efficient dielectric screening and releasing the quantum confinement. Consequently, the optical conductivity and plasmon excitation slightly improve, and the electronic band structures remain unchanged in graphene/h-BN/MoS2, explaining their fascinating optoelectronic responses. Moreover, the excitonic binding energies of graphene/h-BN/MoS2 redshift with respect to the graphene/MoS2 counterparts. Our results, as well as the broadband optical constants, will help better understand the h-BN barrier layers, facilitating the developing progress of h-BN-based tunneling optoelectronic devices. 2022 American Chemical Society.
URL标识查看原文
内容类型期刊论文
源URL[http://ir.ciomp.ac.cn/handle/181722/67056]  
专题中国科学院长春光学精密机械与物理研究所
推荐引用方式
GB/T 7714
X. Zhu,J. He,W. Liu,et al. Revealing the Modulation Effects on the Electronic Band Structures and Exciton Properties by Stacking Graphene/h-BN/MoS2Schottky Heterostructures[J],2022.
APA X. Zhu.,J. He.,W. Liu.,Y. Zheng.,C. Sheng.,...&R. Zhang and J. Chu.(2022).Revealing the Modulation Effects on the Electronic Band Structures and Exciton Properties by Stacking Graphene/h-BN/MoS2Schottky Heterostructures..
MLA X. Zhu,et al."Revealing the Modulation Effects on the Electronic Band Structures and Exciton Properties by Stacking Graphene/h-BN/MoS2Schottky Heterostructures".(2022).
个性服务
查看访问统计
相关权益政策
暂无数据
收藏/分享
所有评论 (0)
暂无评论
 

除非特别说明,本系统中所有内容都受版权保护,并保留所有权利。


©版权所有 ©2017 CSpace - Powered by CSpace