Rapid Detection of Hydrogen Sulfide Gas at Ambient Humidity Based on Nafion-High-Field Asymmetric Waveform Ion Mobility Spectrometry Technology

doi:10.19756/j.issn.0253-3820.221019

	Rapid Detection of Hydrogen Sulfide Gas at Ambient Humidity Based on Nafion-High-Field Asymmetric Waveform Ion Mobility Spectrometry Technology
	Shan, Li 1,2; Zhen, Chen 1,2; Liu, Chang-Jie 2; Jiao, Jin 1,2; Han, Wang 1,2; Jun, Hu 1,2; He, Ma 1,2; Shi, Jia-Liang ; Qian, Ren 3; Cheng, Yu-Peng 1,2
刊名	CHINESE JOURNAL OF ANALYTICAL CHEMISTRY
	2022-06-01
卷号	50
关键词	Hydrogen sulfide High-field asymmetric waveform ion mobility spectrometry Humidity Field detection
ISSN号	0253-3820
DOI	10.19756/j.issn.0253-3820.221019
通讯作者	Liu, You-Jiang() ; Chen, Chi-Lai()
英文摘要	High- field asymmetric waveform ion mobility spectrometry(FAIMS)is a fast and sensitive field detection technology, but the detection of polar substances using FAIMS is easily affected by humidity. Based on that nafion tube could selectively and quickly filter water gas, a nafion- FAIMS technology was proposed for rapid detection of environmental hydrogen sulfide(H2S)gas under ambient humidity in this work. The self- made nafion-FAIMS device was used to study the stability of nafionFAIMS in detection of H2S under different humidity conditions, the separation and identification ability of H2S in the presence of typical environmental interferents, the linearity and the detection limit. The results showed that when the relative humidity was 5%-50%, the relative standard deviations(RSDs)of peak position and peak height of H2S spectrum were less than 0.4% and 0.2%, respectively, which were 10 times and 250 times smaller than that of single FAIMS, showing high recognition and quantitative stability. When the dispersion voltage was 1200 V, the relative deviation of peak height and peak position between benzene and H2S mixed gas spectrum and single substance were only 0.7% and 2%, indicating the adaptability of nafion- FAIMS to mixture detection. The signal linearity reached 98% in the H2S concentration range of 0.08-0.46 mg/m(3), and the detection limit was 0.04 mg/m(3).
资助项目	National Natural Science Foundation of China[61871367] ; National Natural Science Foundation of China[41805017] ; Youth Innovation Promotion Association of Chinese Academy of Sciences[2013213] ; Fundamental Research Funds for the Central Universities[WK5290000002] ; Chinese Academy of Sciences Hefei Institute of Material Science Double Innovation Fund[KY-2021-SC-05]
WOS关键词	UV-FAIMS ; SENSOR
WOS研究方向	Chemistry
语种	英语
出版者	SCIENCE PRESS
WOS记录号	WOS:000884100200015
资助机构	National Natural Science Foundation of China ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; Fundamental Research Funds for the Central Universities ; Chinese Academy of Sciences Hefei Institute of Material Science Double Innovation Fund
内容类型	期刊论文
源URL	[http://ir.hfcas.ac.cn:8080/handle/334002/130156]
专题	中国科学院合肥物质科学研究院
通讯作者	Liu, You-Jiang; Chen, Chi-Lai
作者单位	1.Univ Sci & Technol China, Hefei 230026, Peoples R China 2.Chinese Acad Sci, Hefei Inst Phys Sci, Hefei 230031, Peoples R China 3.INOPEC Beijing Yanshan Co, Beijing 102500, Peoples R China
推荐引用方式 GB/T 7714	Shan, Li,Zhen, Chen,Liu, Chang-Jie,et al. Rapid Detection of Hydrogen Sulfide Gas at Ambient Humidity Based on Nafion-High-Field Asymmetric Waveform Ion Mobility Spectrometry Technology[J]. CHINESE JOURNAL OF ANALYTICAL CHEMISTRY,2022,50.
APA	Shan, Li.,Zhen, Chen.,Liu, Chang-Jie.,Jiao, Jin.,Han, Wang.,...&Chen, Chi-Lai.(2022).Rapid Detection of Hydrogen Sulfide Gas at Ambient Humidity Based on Nafion-High-Field Asymmetric Waveform Ion Mobility Spectrometry Technology.CHINESE JOURNAL OF ANALYTICAL CHEMISTRY,50.
MLA	Shan, Li,et al."Rapid Detection of Hydrogen Sulfide Gas at Ambient Humidity Based on Nafion-High-Field Asymmetric Waveform Ion Mobility Spectrometry Technology".CHINESE JOURNAL OF ANALYTICAL CHEMISTRY 50(2022).