Waste biomass-assisted synthesis of TiO2 and N/O-contained graphene- like biochar composites for enhanced adsorptive and photocatalytic performances | |
Luo, Hao3; Yu, Shunli3; Zhong, Ming1,3; Han, Yuqi2; Su, Bitao3; Lei, Ziqiang3 | |
刊名 | JOURNAL OF ALLOYS AND COMPOUNDS |
2022-04-05 | |
卷号 | 899 |
关键词 | Biomass TiO2 Biochar Characterization Adsorptive and photocatalytic performances |
ISSN号 | 0925-8388 |
DOI | 10.1016/j.jallcom.2021.163287 |
英文摘要 | Titanium dioxide (TiO2) is a promising semiconductor photocatalyst for degradation of organic pollutants but is hampered by bandwidth prohibition and high probability of photo-generated electron-hole recombination. Searching for effective modification strategies to alleviate these issues is thus particularly significant. Herein, two series of composites of TiO2 and graphene-like biochar (PC) were prepared via a simple biomass-assisted pyrolysis coupled with activation strategy and characterized by various techniques. The methylene blue (MB)-simulated waste water was used to evaluate their adsorptive and photocatalytic performances. The results showed that the optimal TiO2-PC composite delivered an excellent photocatalytic performance, nearly 4 times as TiO2. The enhanced performance was probably caused by the synergistic effect among the graphene-like PC, the self-introduced N/O heteroatom, and the interaction between TiO2 and PC. Furthermore, the possible photocatalytic process was also proposed. This work may provide a guidance on preparing high-performance composites through a simple, cheap, and environmental biomass assisted strategy for highly-efficient photocatalysis application. (C) 2021 Elsevier B.V. All rights reserved. |
WOS研究方向 | Chemistry ; Materials Science ; Metallurgy & Metallurgical Engineering |
语种 | 英语 |
出版者 | ELSEVIER SCIENCE SA |
WOS记录号 | WOS:000749614300001 |
内容类型 | 期刊论文 |
源URL | [http://ir.lut.edu.cn/handle/2XXMBERH/154766] |
专题 | 省部共建有色金属先进加工与再利用国家重点实验室 |
作者单位 | 1.Lanzhou Univ Technol, State Key Lab Adv Proc & Recycling Nonferrous Met, Lanzhou 730050, Peoples R China; 2.He Xi Univ, Coll Chem & Chem Engn, Zhangye 734000, Peoples R China 3.Northwest Normal Univ, Coll Chem & Chem Engn, Key Lab Ecoenvironm Polymer Mat Gansu Prov, Minist Educ,Key Lab Ecofunct Polymer Mat, Lanzhou 730070, Peoples R China; |
推荐引用方式 GB/T 7714 | Luo, Hao,Yu, Shunli,Zhong, Ming,et al. Waste biomass-assisted synthesis of TiO2 and N/O-contained graphene- like biochar composites for enhanced adsorptive and photocatalytic performances[J]. JOURNAL OF ALLOYS AND COMPOUNDS,2022,899. |
APA | Luo, Hao,Yu, Shunli,Zhong, Ming,Han, Yuqi,Su, Bitao,&Lei, Ziqiang.(2022).Waste biomass-assisted synthesis of TiO2 and N/O-contained graphene- like biochar composites for enhanced adsorptive and photocatalytic performances.JOURNAL OF ALLOYS AND COMPOUNDS,899. |
MLA | Luo, Hao,et al."Waste biomass-assisted synthesis of TiO2 and N/O-contained graphene- like biochar composites for enhanced adsorptive and photocatalytic performances".JOURNAL OF ALLOYS AND COMPOUNDS 899(2022). |
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