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Controlled Synthesis of Mesoporous CeO2-WO3/TiO2 Microspheres Catalysts for the Selective Catalytic Reduction of NOx with NH3
Guo, Jie1,2; Zhang, Guodong1; Tang, Zhicheng1; Zhang, Jiyi2
刊名CATALYSIS SURVEYS FROM ASIA
2019-12-01
卷号23期号:4页码:311-321
关键词Hydrothermal method Selective catalytic reduction Micro-spheres CeO2-WO3/TiO2 Morphology Mesoporous material
ISSN号1571-1013
DOI10.1007/s10563-019-09278-0
英文摘要A series of mesoporous TiO2 supports were synthesized by changing the hydrothermal temperature. Subsequently, CeO2-WO3/TiO2 catalysts were prepared by impregnation method and applied for selective catalytic reduction (SCR) of NOx with NH3. In addition, the morphology of TiO2 changed from microspheres to ellipsoidal microspheres by gradually increasing the hydrothermal temperature which was 120 degrees C, 160 degrees C and 200 degrees C. Obviously, the SCR activity was exhibited in the following order: CeO2-WO3/TiO2-160 > CeO2-WO3/TiO2-120 > CeO2-WO3/TiO2-200. Among, the CeO2-WO3/TiO2-160 catalyst exhibited better catalytic activity for the NH3-SCR reaction. Through a series of characterizations, it was concluded that the mesoporous structure, redox ability and abundant surface acidity of the CeO2-WO3/TiO2 catalyst played a critical role in improving the activity, resistant of H2O and SO2.
WOS研究方向Chemistry
语种英语
出版者SPRINGER/PLENUM PUBLISHERS
WOS记录号WOS:000519782800005
内容类型期刊论文
源URL[http://ir.lut.edu.cn/handle/2XXMBERH/155285]  
专题石油化工学院
作者单位1.Chinese Acad Sci, State Key Lab Oxo Synth & Select Oxidat, Natl Engn Res Ctr Fine Petrochem Intermediates, Lanzhou Inst Chem Phys, Lanzhou 730000, Peoples R China;
2.Lanzhou Univ Technol, Sch Petr & Chem, Lanzhou 730050, Peoples R China
推荐引用方式
GB/T 7714
Guo, Jie,Zhang, Guodong,Tang, Zhicheng,et al. Controlled Synthesis of Mesoporous CeO2-WO3/TiO2 Microspheres Catalysts for the Selective Catalytic Reduction of NOx with NH3[J]. CATALYSIS SURVEYS FROM ASIA,2019,23(4):311-321.
APA Guo, Jie,Zhang, Guodong,Tang, Zhicheng,&Zhang, Jiyi.(2019).Controlled Synthesis of Mesoporous CeO2-WO3/TiO2 Microspheres Catalysts for the Selective Catalytic Reduction of NOx with NH3.CATALYSIS SURVEYS FROM ASIA,23(4),311-321.
MLA Guo, Jie,et al."Controlled Synthesis of Mesoporous CeO2-WO3/TiO2 Microspheres Catalysts for the Selective Catalytic Reduction of NOx with NH3".CATALYSIS SURVEYS FROM ASIA 23.4(2019):311-321.
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