Visible light-driven photocatalytic degradation of organic pollutants via carbon quantum dots/TiO2 | |
Wang, Kunjie1,2; Liang, Lei2; Zheng, Yi2; Li, Hongxia2; Niu, Xiaohui2; Zhang, Deyi2; Fan, Haiyan3 | |
刊名 | NEW JOURNAL OF CHEMISTRY |
2021-09-21 | |
卷号 | 45期号:35页码:16168-16178 |
ISSN号 | 1144-0546 |
DOI | 10.1039/d1nj02387j |
英文摘要 | Using olive leaves as the carbon source, carbon quantum dots (CQDs) with up-conversion luminescence were prepared via a reflux method. Through a hydrothermal treatment, CQDs were loaded on the surface of TiO2 to form a CQDs/TiO2 composite that exhibited photocatalytic properties. The morphology, size and composition of the as-prepared composite were characterized using XRD, SEM, TEM and XPS. Excited at the wavelength range from 560 nm to 740 nm, CQDs exhibited a significant multi-photon-based up-conversion luminescence property. This property of CQDs endowed CQDs/TiO2 composites with great photocatalytic efficiency. The performance of CQDs/TiO2 composites was tested in the degradation of tetracycline (TC) and rhodamine B (RhB). Irradiated under visible light for 10 min and 70 min, the degradation rates of 5% CQDs/TiO2 reached 81% and 92% for TC and RhB, respectively. Photocurrent and PL tests indicated that the loading of CQDs significantly improved the separation efficiency of TiO2-photogenerated charge carriers. Taking advantage of the up-conversion luminescence property of CQDs, the harvesting efficiency of visible light by CQDs/TiO2 composites was greatly enhanced. |
WOS研究方向 | Chemistry |
语种 | 英语 |
出版者 | ROYAL SOC CHEMISTRY |
WOS记录号 | WOS:000686744400001 |
内容类型 | 期刊论文 |
源URL | [http://ir.lut.edu.cn/handle/2XXMBERH/148932] |
专题 | 石油化工学院 |
作者单位 | 1.Lanzhou Univ Technol, Sch Petrochem Technol, Lanzhou 730050, Peoples R China; 2.Key Lab Low Carbon Energy & Chem Engn Gansu Prov, Lanzhou 730050, Peoples R China; 3.Nazarbayev Univ, Chem Dept, Astana 010000, Kazakhstan |
推荐引用方式 GB/T 7714 | Wang, Kunjie,Liang, Lei,Zheng, Yi,et al. Visible light-driven photocatalytic degradation of organic pollutants via carbon quantum dots/TiO2[J]. NEW JOURNAL OF CHEMISTRY,2021,45(35):16168-16178. |
APA | Wang, Kunjie.,Liang, Lei.,Zheng, Yi.,Li, Hongxia.,Niu, Xiaohui.,...&Fan, Haiyan.(2021).Visible light-driven photocatalytic degradation of organic pollutants via carbon quantum dots/TiO2.NEW JOURNAL OF CHEMISTRY,45(35),16168-16178. |
MLA | Wang, Kunjie,et al."Visible light-driven photocatalytic degradation of organic pollutants via carbon quantum dots/TiO2".NEW JOURNAL OF CHEMISTRY 45.35(2021):16168-16178. |
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