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Visible light-driven photocatalytic degradation of organic pollutants via carbon quantum dots/TiO2
Wang, Kunjie1,2; Liang, Lei2; Zheng, Yi2; Li, Hongxia2; Niu, Xiaohui2; Zhang, Deyi2; Fan, Haiyan3
刊名NEW JOURNAL OF CHEMISTRY
2021-09-21
卷号45期号:35页码:16168-16178
ISSN号1144-0546
DOI10.1039/d1nj02387j
英文摘要Using olive leaves as the carbon source, carbon quantum dots (CQDs) with up-conversion luminescence were prepared via a reflux method. Through a hydrothermal treatment, CQDs were loaded on the surface of TiO2 to form a CQDs/TiO2 composite that exhibited photocatalytic properties. The morphology, size and composition of the as-prepared composite were characterized using XRD, SEM, TEM and XPS. Excited at the wavelength range from 560 nm to 740 nm, CQDs exhibited a significant multi-photon-based up-conversion luminescence property. This property of CQDs endowed CQDs/TiO2 composites with great photocatalytic efficiency. The performance of CQDs/TiO2 composites was tested in the degradation of tetracycline (TC) and rhodamine B (RhB). Irradiated under visible light for 10 min and 70 min, the degradation rates of 5% CQDs/TiO2 reached 81% and 92% for TC and RhB, respectively. Photocurrent and PL tests indicated that the loading of CQDs significantly improved the separation efficiency of TiO2-photogenerated charge carriers. Taking advantage of the up-conversion luminescence property of CQDs, the harvesting efficiency of visible light by CQDs/TiO2 composites was greatly enhanced.
WOS研究方向Chemistry
语种英语
出版者ROYAL SOC CHEMISTRY
WOS记录号WOS:000686744400001
内容类型期刊论文
源URL[http://ir.lut.edu.cn/handle/2XXMBERH/148932]  
专题石油化工学院
作者单位1.Lanzhou Univ Technol, Sch Petrochem Technol, Lanzhou 730050, Peoples R China;
2.Key Lab Low Carbon Energy & Chem Engn Gansu Prov, Lanzhou 730050, Peoples R China;
3.Nazarbayev Univ, Chem Dept, Astana 010000, Kazakhstan
推荐引用方式
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Wang, Kunjie,Liang, Lei,Zheng, Yi,et al. Visible light-driven photocatalytic degradation of organic pollutants via carbon quantum dots/TiO2[J]. NEW JOURNAL OF CHEMISTRY,2021,45(35):16168-16178.
APA Wang, Kunjie.,Liang, Lei.,Zheng, Yi.,Li, Hongxia.,Niu, Xiaohui.,...&Fan, Haiyan.(2021).Visible light-driven photocatalytic degradation of organic pollutants via carbon quantum dots/TiO2.NEW JOURNAL OF CHEMISTRY,45(35),16168-16178.
MLA Wang, Kunjie,et al."Visible light-driven photocatalytic degradation of organic pollutants via carbon quantum dots/TiO2".NEW JOURNAL OF CHEMISTRY 45.35(2021):16168-16178.
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