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Synthesis of a Novel CQDs-GO-Ag2S Composite and Study on the Adsorption of Methylene Blue
Zhang, Dongqiang, I1; Xu, Jialin1; Liang, Lei1; Li, Hongxia1; Du, Mei1; Liu, Xiaoyu1; Wang, Kunjie1,2
刊名CHEMISTRYSELECT
2020-02-28
卷号5期号:8页码:2501-2507
关键词Adsorption Carbon dots Composite materials GO
ISSN号2365-6549
DOI10.1002/slct.202000102
英文摘要The present work aims to develop a composite that takes the advantages of carbon quantum dots (CQDs) such as wide absorption band, high optical absorption coefficient and chemical stability as well as the nano-sized silver sulfide with excellent redox capacity and the strong absorption in the visible range. Such nanocomposites were crafted on a template developed using polyethyleneimine (PEI) modified Graphene oxide (GO). The adsorption properties of methylene blue dyes were tested. With the large specific surface area, the as prepared nanocomposites achieved the removal rate of the blue dye up to 99.0%. The adsorption process was able to be described using the Freundlich isothermal model, wherein, the maximum adsorption capacity was obtained as 348 mg.g(-1). Thermodynamic analysis indicates the adsorption is entropy driven process with Delta G < 0, Delta H > 0, and Delta S > 0. The present study shows that CQDs-GO-Ag2S composites as a promising adsorbent that may be applied to wastewater treatment and waste gas removal.
资助项目National Natural Science Foundation of China Project[21867015][31860250]
WOS研究方向Chemistry
语种英语
出版者WILEY-V C H VERLAG GMBH
WOS记录号WOS:000516865300021
状态已发表
内容类型期刊论文
源URL[http://ir.lut.edu.cn/handle/2XXMBERH/64148]  
专题石油化工学院
通讯作者Wang, Kunjie
作者单位1.Lanzhou Univ Technol, Coll Petrochem Technol, Lanzhou 730050, Gansu, Peoples R China
2.Minist Educ, Key Lab Ecofunct Polymer Mat, Lanzhou 730070, Gansu, Peoples R China
推荐引用方式
GB/T 7714
Zhang, Dongqiang, I,Xu, Jialin,Liang, Lei,et al. Synthesis of a Novel CQDs-GO-Ag2S Composite and Study on the Adsorption of Methylene Blue[J]. CHEMISTRYSELECT,2020,5(8):2501-2507.
APA Zhang, Dongqiang, I.,Xu, Jialin.,Liang, Lei.,Li, Hongxia.,Du, Mei.,...&Wang, Kunjie.(2020).Synthesis of a Novel CQDs-GO-Ag2S Composite and Study on the Adsorption of Methylene Blue.CHEMISTRYSELECT,5(8),2501-2507.
MLA Zhang, Dongqiang, I,et al."Synthesis of a Novel CQDs-GO-Ag2S Composite and Study on the Adsorption of Methylene Blue".CHEMISTRYSELECT 5.8(2020):2501-2507.
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