Synthesis of a Novel CQDs-GO-Ag2S Composite and Study on the Adsorption of Methylene Blue | |
Zhang, Dongqiang, I1; Xu, Jialin1; Liang, Lei1; Li, Hongxia1; Du, Mei1; Liu, Xiaoyu1; Wang, Kunjie1,2 | |
刊名 | CHEMISTRYSELECT |
2020-02-28 | |
卷号 | 5期号:8页码:2501-2507 |
关键词 | Adsorption Carbon dots Composite materials GO |
ISSN号 | 2365-6549 |
DOI | 10.1002/slct.202000102 |
英文摘要 | The present work aims to develop a composite that takes the advantages of carbon quantum dots (CQDs) such as wide absorption band, high optical absorption coefficient and chemical stability as well as the nano-sized silver sulfide with excellent redox capacity and the strong absorption in the visible range. Such nanocomposites were crafted on a template developed using polyethyleneimine (PEI) modified Graphene oxide (GO). The adsorption properties of methylene blue dyes were tested. With the large specific surface area, the as prepared nanocomposites achieved the removal rate of the blue dye up to 99.0%. The adsorption process was able to be described using the Freundlich isothermal model, wherein, the maximum adsorption capacity was obtained as 348 mg.g(-1). Thermodynamic analysis indicates the adsorption is entropy driven process with Delta G < 0, Delta H > 0, and Delta S > 0. The present study shows that CQDs-GO-Ag2S composites as a promising adsorbent that may be applied to wastewater treatment and waste gas removal. |
资助项目 | National Natural Science Foundation of China Project[21867015][31860250] |
WOS研究方向 | Chemistry |
语种 | 英语 |
出版者 | WILEY-V C H VERLAG GMBH |
WOS记录号 | WOS:000516865300021 |
状态 | 已发表 |
内容类型 | 期刊论文 |
源URL | [http://ir.lut.edu.cn/handle/2XXMBERH/64148] |
专题 | 石油化工学院 |
通讯作者 | Wang, Kunjie |
作者单位 | 1.Lanzhou Univ Technol, Coll Petrochem Technol, Lanzhou 730050, Gansu, Peoples R China 2.Minist Educ, Key Lab Ecofunct Polymer Mat, Lanzhou 730070, Gansu, Peoples R China |
推荐引用方式 GB/T 7714 | Zhang, Dongqiang, I,Xu, Jialin,Liang, Lei,et al. Synthesis of a Novel CQDs-GO-Ag2S Composite and Study on the Adsorption of Methylene Blue[J]. CHEMISTRYSELECT,2020,5(8):2501-2507. |
APA | Zhang, Dongqiang, I.,Xu, Jialin.,Liang, Lei.,Li, Hongxia.,Du, Mei.,...&Wang, Kunjie.(2020).Synthesis of a Novel CQDs-GO-Ag2S Composite and Study on the Adsorption of Methylene Blue.CHEMISTRYSELECT,5(8),2501-2507. |
MLA | Zhang, Dongqiang, I,et al."Synthesis of a Novel CQDs-GO-Ag2S Composite and Study on the Adsorption of Methylene Blue".CHEMISTRYSELECT 5.8(2020):2501-2507. |
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