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Biomass derived porous carbon for efficient capture of carbon dioxide, organic contaminants and volatile iodine with exceptionally high uptake
Sun, Hanxue1; Yang, Boli2; Li, An1
刊名CHEMICAL ENGINEERING JOURNAL
2019-09-15
卷号372页码:65-73
关键词Porous carbon Sunflowers Iodine capture Biomass
ISSN号1385-8947
DOI10.1016/j.cej.2019.04.061
英文摘要Environmentally sustainable development and concerns have increased interested in biomass materials for synthesis of porous carbons, especially as effectively alternative and multifunctional sorbents for diverse contaminates and in CO2 adsorption area. In this work, spongy flesh from receptacle and stalk of sunflowers was utilized as carbonaceous precursors to prepare porous carbons by pyrolysis method with and without KOH activation in argon. The biomass-derived porous carbon has high surface area (up to 3072 m(2) g(-1)), light bulk density (0.033 g cm(-3)) and different morphology depending on the preparation method. Taking advantages of the highly porosity and the valuable hierarchical porous structure, the resulting porous carbons can serve well as multifunctional solid sorbents for CO2, radioactive iodine and oily/organic contaminates from water. In particular, the resulting carbon sample shows a high iodine affinity with an uptake of 646 wt%, which is the highest value reported to date. Given the worldwide abundance and recyclability, spongy flesh from receptacle and stalk of sunflowers can be serve as a new biomass source for the facile production of high-performance porous carbon materials with promising applications in environmental remediation.
资助项目National Natural Science Foundation of China[51663012][51462021] ; Support Program for Hongliu Young Teachers of LUT, Collaborative Innovation Team, Gansu Province, China[052005] ; Innovation and Entrepreneurship Talent Project of Lanzhou[2017-RC-33]
WOS研究方向Engineering
语种英语
出版者ELSEVIER SCIENCE SA
WOS记录号WOS:000471670400007
状态已发表
内容类型期刊论文
源URL[http://119.78.100.223/handle/2XXMBERH/31570]  
专题石油化工学院
通讯作者Li, An
作者单位1.Lanzhou Univ Technol, Coll Petrochem Engn, Dept Chem Engn, Lanzhou 730050, Gansu, Peoples R China
2.CCDC Changqing Downhole Technol Co, Xian 710018, Shaanxi, Peoples R China
推荐引用方式
GB/T 7714
Sun, Hanxue,Yang, Boli,Li, An. Biomass derived porous carbon for efficient capture of carbon dioxide, organic contaminants and volatile iodine with exceptionally high uptake[J]. CHEMICAL ENGINEERING JOURNAL,2019,372:65-73.
APA Sun, Hanxue,Yang, Boli,&Li, An.(2019).Biomass derived porous carbon for efficient capture of carbon dioxide, organic contaminants and volatile iodine with exceptionally high uptake.CHEMICAL ENGINEERING JOURNAL,372,65-73.
MLA Sun, Hanxue,et al."Biomass derived porous carbon for efficient capture of carbon dioxide, organic contaminants and volatile iodine with exceptionally high uptake".CHEMICAL ENGINEERING JOURNAL 372(2019):65-73.
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