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The effect of temperatures on the synergistic effect between a magnetic field and functionalized graphene oxide-carbon nanotube composite for Pb2+ and phenol adsorption
Jiang, Li-li1; Yu, Hai-Tao2; Pei, Lie-fei1; Hou, Xin-gang1
刊名Journal of Nanomaterials
2018
卷号2018
关键词Activation energy Adsorption Graphene Magnetic fields Multiwalled carbon nanotubes (MWCN) Nanotubes Phenols Water treatment Adsorption properties Effect of temperature Freundlich isotherm model Functionalized graphene Increased temperature Increasing temperatures Intramolecular energy Pseudo-second-order kinetic models
ISSN号16874110
DOI10.1155/2018/9167938
英文摘要The effect of temperature on scale inhibition and adsorption properties for Pb2+ and phenol was studied under the synergistic effect of the magnetic field and the adsorbent. The sulfhydryl and amino-modified graphene oxide/oxidized multiwalled carbon nanotubes (NH2-SH-GO/o-MWCNTs) were synthesized and applied as the adsorbent. Additionally, changes in pH, conductivity, molecular activation energy, the relative variation of intramolecular energy and the relative variation in the proportion of free water, and adsorption capacity of the adsorbent were studied under different temperatures of circulating water. The relative variation of the proportion of free water increased with the increasing temperatures. The above results indicated that higher temperature would be detrimental to scale inhibition. The higher the temperatures, the lower the intramolecular energies. And the more stable molecules are formed in the circulating water. Thus, the results reduced the tendency to scale formation. The increased temperatures promoted the adsorption capacity of the adsorbent for Pb2+ and phenol. The adsorption process for Pb2+ and phenol conformed to the pseudo-second-order kinetic model and Freundlich isotherm model under the synergistic effect of magnetic field and NH2-SH-GO/MWCNTs. After five cycles, the adsorption capacities of the adsorbent for Pb2+ and phenol separately decreased by 59.86% and 76.36%. The aforementioned results reveal that temperatures can promote the adsorption process for Pb2+ and phenol, and the synergistic effect between magnetic field and the adsorbent has a potential application for water treatment. © 2018 Li-li Jiang et al.
资助项目Lanzhou University of Technology[061702]
WOS研究方向Science & Technology - Other Topics ; Materials Science
语种英语
出版者Hindawi Limited, 410 Park Avenue, 15th Floor, 287 pmb, New York, NY 10022, United States
WOS记录号WOS:000441599900001
状态已发表
内容类型期刊论文
源URL[http://ir.lut.edu.cn/handle/2XXMBERH/114471]  
专题材料科学与工程学院
通讯作者Jiang, Li-li
作者单位1.Lanzhou Univ Technol, Sch Mat Sci & Technol, Langongping Rd, Lanzhou 730050, Gansu, Peoples R China
2.Lanzhou Univ, Hosp 1, Dept Med Lab, 1 Donggang Rd, Lanzhou 730000, Gansu, Peoples R China
推荐引用方式
GB/T 7714
Jiang, Li-li,Yu, Hai-Tao,Pei, Lie-fei,et al. The effect of temperatures on the synergistic effect between a magnetic field and functionalized graphene oxide-carbon nanotube composite for Pb2+ and phenol adsorption[J]. Journal of Nanomaterials,2018,2018.
APA Jiang, Li-li,Yu, Hai-Tao,Pei, Lie-fei,&Hou, Xin-gang.(2018).The effect of temperatures on the synergistic effect between a magnetic field and functionalized graphene oxide-carbon nanotube composite for Pb2+ and phenol adsorption.Journal of Nanomaterials,2018.
MLA Jiang, Li-li,et al."The effect of temperatures on the synergistic effect between a magnetic field and functionalized graphene oxide-carbon nanotube composite for Pb2+ and phenol adsorption".Journal of Nanomaterials 2018(2018).
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