Novel MOF-Based Photocatalyst AgBr/AgCl@ZIF-8 with Enhanced Photocatalytic Degradation and Antibacterial Properties
Liu, Ning1,2,3; Zhang, Jie1,3; Wang, Yanhua2; Zhu, Qingjun1,3; Zhang, Xuan2; Duan, Jizhou1,3; Hou, Baorong1,3
刊名NANOMATERIALS
2022-06-01
卷号12期号:11页码:13
关键词photocatalysis metal-organic frameworks photocatalytic antibacterial organic pollutants
DOI10.3390/nano12111946
通讯作者Zhang, Jie(zhangjie@qdio.ac.cn) ; Wang, Yanhua(wyhazz@163.com)
英文摘要A novel visible light-driven AgBr/AgCl@ZIF-8 catalyst was synthesized by a simple and rapid method. The composition and structure of the photocatalyst were characterized by XRD, SEM, UV-DRS, and XPS. It could be observed that the 2-methylimidazole zinc salt (ZIF-8) exhibited the rhombic dodecahedron morphology with the AgCl and AgBr particles evenly distributed around it. The composite photocatalyst AgBr/AgCl@ZIF-8 showed good photocatalytic degradation and antibacterial properties. The degradation rate of RhB solution was 98%, with 60 min of irradiation of visible light, and almost all P. aeruginosaudomonas aeruginosa (P. aeruginosa), Staphylococcus aureus (S. aureus), and Escherichia coli (E. coli) were inactivated under the irradiation of 90 min. In addition, the prepared catalyst had excellent stability and reusability. Based on the free radical capture experiment, center dot O-2(-) and h(+) were believed to be the main active substances, and possible photocatalytic degradation and sterilization mechanisms of AgBr/AgCl@ZIF-8 were proposed.
资助项目National Natural Science Foundation of China[42076043] ; Shandong Provincial Natural Science Foundation[ZR2020MD080]
WOS研究方向Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
语种英语
出版者MDPI
WOS记录号WOS:000808931300001
内容类型期刊论文
源URL[http://ir.qdio.ac.cn/handle/337002/179443]  
专题海洋研究所_海洋腐蚀与防护研究发展中心
通讯作者Zhang, Jie; Wang, Yanhua
作者单位1.Chinese Acad Sci, Inst Oceanol, Key Lab Marine Environm Corros & Biofouling, Qingdao 266071, Peoples R China
2.Ocean Univ China, Coll Chem & Chem Engn, Key Lab Marine Chem Theory & Technol, Minist Educ, Qingdao 266100, Peoples R China
3.Pilot Natl Lab Marine Sci & Technol Qingdao, Open Studio Marine Corros & Protect, 1 Wenhai Rd, Qingdao 266237, Peoples R China
推荐引用方式
GB/T 7714
Liu, Ning,Zhang, Jie,Wang, Yanhua,et al. Novel MOF-Based Photocatalyst AgBr/AgCl@ZIF-8 with Enhanced Photocatalytic Degradation and Antibacterial Properties[J]. NANOMATERIALS,2022,12(11):13.
APA Liu, Ning.,Zhang, Jie.,Wang, Yanhua.,Zhu, Qingjun.,Zhang, Xuan.,...&Hou, Baorong.(2022).Novel MOF-Based Photocatalyst AgBr/AgCl@ZIF-8 with Enhanced Photocatalytic Degradation and Antibacterial Properties.NANOMATERIALS,12(11),13.
MLA Liu, Ning,et al."Novel MOF-Based Photocatalyst AgBr/AgCl@ZIF-8 with Enhanced Photocatalytic Degradation and Antibacterial Properties".NANOMATERIALS 12.11(2022):13.
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