Spatially Separated Photosystem II and a Silicon Photoelectrochemical Cell for Overall Water Splitting: A Natural-Artificial Photosynthetic Hybrid

doi:10.1002/anie.201604091

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	Spatially Separated Photosystem II and a Silicon Photoelectrochemical Cell for Overall Water Splitting: A Natural-Artificial Photosynthetic Hybrid
	Wang, Wangyin ; Wang, Hong 4; Zhu, Qingjun 4; Qin, Wei ; Han, Guangye ; Shen, Jian-Ren ; Zong, Xu ; Li, Can
刊名	ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
	2016
卷号	55 期号:32 页码:9229-9233
关键词	photocatalysis photoelectrochemistry photosystem II water splitting Z-scheme
ISSN号	1433-7851
DOI	10.1002/anie.201604091
文献子类	Article
英文摘要	Integrating natural and artificial photosynthetic platforms is an important approach to developing solar-driven hybrid systems with exceptional function over the individual components. A natural-artificial photosynthetic hybrid platform is formed by wiring photosystem II (PSII) and a platinum-decorated silicon photoelectrochemical (PEC) cell in a tandem manner based on a photocatalytic-PEC Z-scheme design. Although the individual components cannot achieve overall water splitting, the hybrid platform demonstrated the capability of unassisted solar-driven overall water splitting. Moreover, H-2 and O-2 evolution can be separated in this system, which is ascribed to the functionality afforded by the unconventional Z-scheme design. Furthermore, the tandem configuration and the spatial separation between PSII and artificial components provide more opportunities to develop efficient natural-artificial hybrid photosynthesis systems.
学科主题	Chemistry, Multidisciplinary
电子版国际标准刊号	1521-3773
出版地	WEINHEIM
WOS关键词	PHOTO-BIOELECTROCHEMICAL CELLS ; SHUTTLE REDOX MEDIATOR ; VISIBLE-LIGHT ; ELECTRON-TRANSFER ; Z-SCHEME ; OXYGEN ; SOLAR ; PHOTOCATALYSTS ; SYSTEM ; RESOLUTION
WOS研究方向	Science Citation Index Expanded (SCI-EXPANDED)
语种	英语
出版者	WILEY-V C H VERLAG GMBH
WOS记录号	WOS:000383371800017
资助机构	973 National Basic Research Program of the Ministry of Science and TechnologyNational Basic Research Program of China [2014CB239403] ; National Natural Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [21090340] ; Key Research Program of the Chinese Academy of Science [KGZD-EW-T05] ; Young Thousand Talents Program of China
内容类型	期刊论文
源URL	[http://ir.ibcas.ac.cn/handle/2S10CLM1/25304]
专题	中科院光生物学重点实验室
作者单位	1.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 2.Chinese Acad Sci, Inst Bot, Key Lab Photobiol, Photosynthesis Res Ctr, Beijing 100093, Peoples R China 3.Okayama Univ, Grad Sch Nat Sci & Technol, Photosynthesis Res Ctr, 1-1 Naka 3 Chome, Okayama 7008530, Japan 4.Chinese Acad Sci, Collaborat Innovat Ctr Chem Energy Mat IChEM, Dalian Natl Lab Clean Energy, State Key Lab Catalysis,Dalian Inst Chem Phys, Zhongshan Rd 457, Dalian 116023, Peoples R China
推荐引用方式 GB/T 7714	Wang, Wangyin,Wang, Hong,Zhu, Qingjun,et al. Spatially Separated Photosystem II and a Silicon Photoelectrochemical Cell for Overall Water Splitting: A Natural-Artificial Photosynthetic Hybrid[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,2016,55(32):9229-9233.
APA	Wang, Wangyin.,Wang, Hong.,Zhu, Qingjun.,Qin, Wei.,Han, Guangye.,...&Li, Can.(2016).Spatially Separated Photosystem II and a Silicon Photoelectrochemical Cell for Overall Water Splitting: A Natural-Artificial Photosynthetic Hybrid.ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,55(32),9229-9233.
MLA	Wang, Wangyin,et al."Spatially Separated Photosystem II and a Silicon Photoelectrochemical Cell for Overall Water Splitting: A Natural-Artificial Photosynthetic Hybrid".ANGEWANDTE CHEMIE-INTERNATIONAL EDITION 55.32(2016):9229-9233.