Recent progress and prospect of carbon-free single-site catalysts for the hydrogen and oxygen evolution reactions | |
J. Q. Guan; X. Bai and T. M. Tang | |
刊名 | Nano Research |
2022 | |
卷号 | 15期号:2页码:818-837 |
ISSN号 | 1998-0124 |
DOI | 10.1007/s12274-021-3680-9 |
英文摘要 | The key challenge for scalable production of hydrogen from water lies in the rational design and preparation of high-performance and earth-abundant electrocatalysts to replace precious metal Pt and IrO2 for hydrogen evolution reaction (HER) and oxygen evolution reaction (OER). Although atomic M-N-C materials have been extensively studied in heterogeneous catalysis field, the insufficient antioxidant capacity of carbonous substrates hinders their practical application in OER. Developing highly active and stable OER electrocatalysts is the key for electrochemical water splitting. This review presents feasible design strategies for fabricating carbon-free single-site catalysts and their applications in HER/OER and overall water splitting. The constitutive relationships between structure, composition, and catalytic performance for HER and OER are detailly discussed, providing ponderable insights into rationally constructing high-performance HER and OER electrocatalysts. The perspectives on the challenges and future research orientations in single-site catalysts for electrochemical water splitting are suggested. |
URL标识 | 查看原文 |
内容类型 | 期刊论文 |
源URL | [http://ir.ciomp.ac.cn/handle/181722/65577] |
专题 | 中国科学院长春光学精密机械与物理研究所 |
推荐引用方式 GB/T 7714 | J. Q. Guan,X. Bai and T. M. Tang. Recent progress and prospect of carbon-free single-site catalysts for the hydrogen and oxygen evolution reactions[J]. Nano Research,2022,15(2):818-837. |
APA | J. Q. Guan,&X. Bai and T. M. Tang.(2022).Recent progress and prospect of carbon-free single-site catalysts for the hydrogen and oxygen evolution reactions.Nano Research,15(2),818-837. |
MLA | J. Q. Guan,et al."Recent progress and prospect of carbon-free single-site catalysts for the hydrogen and oxygen evolution reactions".Nano Research 15.2(2022):818-837. |
个性服务 |
查看访问统计 |
相关权益政策 |
暂无数据 |
收藏/分享 |
除非特别说明,本系统中所有内容都受版权保护,并保留所有权利。
修改评论