Hematite photoanode modified with inexpensive hole-storage layer for highly efficient solar water oxidation | |
He, Xiaolin5; Shang CQ(商超群)5; Chen ZH(陈志鸿)1,2,3; Jin, Mingliang3,5; Shui, Lingling5; Zhang YG(张永光)3; Zhang, Zhang3,5; Yuan MZ(苑明哲)2; Wang, Xin3,5; Kempa, Krzysztof4 | |
刊名 | Nanotechnology |
2020 | |
卷号 | 31期号:45页码:1-9 |
关键词 | hematite ferrhydrite hole-storage layer photoanode solar water oxidation |
ISSN号 | 0957-4484 |
产权排序 | 2 |
英文摘要 | Hematite is recognized as an excellent photocatalyst for photoelectrochemical photoanodes for water oxidation because of its favorable band gap, excellent anti-photocorrosion and structural stability in alkaline solution. However, slow charge transport and fast carrier recombination in the bulk and at the hematite photoanode/electrolyte interface, have limited its applications for water splitting. Herein, we report a highly efficient hematite/ferrhydrite (Fh) core-shell photoanode system, consisting of hematite (α-Fe2O3) semiconductor nanorods which dramatically enhance light harvesting, and ferrhydrite as the hole-storage shell. Our integrated hematite/ferrhydrite core-shell photoanode shows 2.7 times increased photo-current density under simulated sun light irradiation. © 2020 IOP Publishing Ltd. |
资助项目 | National Natural Science Foundation of China Program[51602111] ; Xijiang RD Team ; Guangdong Innovative and Entrepreneurial Team Program[2016ZT06C517] ; Special Fund Project of Science and Technology Application in Guangdong[2017B020240002] ; Science and Technology Program of Guangzhou[2019050001] ; National 111 project |
WOS关键词 | TANTALUM NITRIDE PHOTOANODE ; NANOROD ARRAYS ; GOLD NANOPARTICLES ; FERRIHYDRITE ; ALPHA-FE2O3 ; ENHANCEMENT ; CATALYST ; NANOTUBE ; FILMS |
WOS研究方向 | Science & Technology - Other Topics ; Materials Science ; Physics |
语种 | 英语 |
WOS记录号 | WOS:000571037200001 |
资助机构 | National Natural Science Foundation of China Program (No.51602111), Xijiang R&D Team (X.W.) ; Guangdong Innovative and Entrepreneurial Team Program (No. 2016ZT06C517) ; Special Fund Project of Science and Technology Application in Guangdong (2017B020240002) ; Science and Technology Program of Guangzhou (2019050001) ; National 111 project |
内容类型 | 期刊论文 |
源URL | [http://ir.sia.cn/handle/173321/27635] |
专题 | 沈阳自动化研究所_广州中国科学院沈阳自动化研究所分所 |
通讯作者 | Chen ZH(陈志鸿); Wang, Xin |
作者单位 | 1.Key Laboratory for Water Quality and Conservation of the Pearl River Delta, Ministry of Education, Institute of Environmental Research at Greater Bay, Guangzhou University, Guangzhou 2.Shenyang Institute of Automation, Chinese Academy of Sciences Guangzhou, Province, Guangzhou, Guangdong, China 3.International Academy of Optoelectronics at Zhaoqing, South China Normal University, China 4.Department of Physics, Boston College, MA 02467, United States 5.Guangdong Provincial Key Laboratory of Optical Information Materials and Technology, South China Academy of Advanced Optoelectronics, South China Normal University, Guangzhou 510006, China |
推荐引用方式 GB/T 7714 | He, Xiaolin,Shang CQ,Chen ZH,et al. Hematite photoanode modified with inexpensive hole-storage layer for highly efficient solar water oxidation[J]. Nanotechnology,2020,31(45):1-9. |
APA | He, Xiaolin.,Shang CQ.,Chen ZH.,Jin, Mingliang.,Shui, Lingling.,...&Zhou, Guofu.(2020).Hematite photoanode modified with inexpensive hole-storage layer for highly efficient solar water oxidation.Nanotechnology,31(45),1-9. |
MLA | He, Xiaolin,et al."Hematite photoanode modified with inexpensive hole-storage layer for highly efficient solar water oxidation".Nanotechnology 31.45(2020):1-9. |
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