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Benzenesulfonic acid-based hydrotropic system for achieving lignocellulose separation and utilization under mild conditions
Dong, Maolin1,2; Wu, Chen1,2; Chen, Lidong1,2; Zhou, Xuelian1,2; Yang, Weisheng4; Xiao, Huining6; Ji, Xingxiang3; Dai, Hongqi1,2; Hu, Chaoquan4,5; Bian, Huiyang1,2,3
刊名BIORESOURCE TECHNOLOGY
2021-10-01
卷号337页码:7
关键词Benzenesulfonic acid Lignocellulose separation and utilization Enzymatic saccharification Lignocellulosic nanofibrils Lignin nanoparticles
ISSN号0960-8524
DOI10.1016/j.biortech.2021.125379
英文摘要Developing low-cost and sustainable fractionation technology is the key to achieve the maximal utilization of lignocellulosic biomass. This study reported benzenesulfonic acid (BA) as a green hydrotrope for efficient lignocellulose conversion into two fractions at atmospheric pressure: (1) a primarily cellulosic solid residue that can be utilized to produce high-value building blocks (lignocellulosic nanomaterials or sugars), and (2) the collected spent acid liquor that can be diluted with anti-solvent to easily obtain lignin nanoparticles. BA hydrotropic method exhibited greater reaction selectivity to solubilize lignin, where approximately 80% lignin were removed at only 80 degrees C in 20 min. The lower lignin content substrates resulted in relatively higher enzymatic hydrolysis efficiency of 80% and less entangled lignocellulosic nanofibrils (LCNF). Furthermore, the separated lignin particles size can be easily adjusted by the initial acid concentration. Overall, this work presented a promising and simple technology in achieving lignocellulose separation and utilization under mild conditions.
资助项目Nanjing IPE Institute of Green Manufacturing Industry[YFW2020071] ; Foundation of State Key Laboratory of Biobased Material and Green Papermaking, Qilu University of Technology[KF201917] ; National College Students Innovation and Entrepreneurship Training Program[201910298155H] ; Shandong Academy of Sciences
WOS关键词FRACTIONATION ; BIOMASS ; WOOD
WOS研究方向Agriculture ; Biotechnology & Applied Microbiology ; Energy & Fuels
语种英语
出版者ELSEVIER SCI LTD
WOS记录号WOS:000684298200007
资助机构Nanjing IPE Institute of Green Manufacturing Industry ; Foundation of State Key Laboratory of Biobased Material and Green Papermaking, Qilu University of Technology ; National College Students Innovation and Entrepreneurship Training Program ; Shandong Academy of Sciences
内容类型期刊论文
源URL[http://ir.ipe.ac.cn/handle/122111/49850]  
专题中国科学院过程工程研究所
通讯作者Bian, Huiyang
作者单位1.Nanjing Forestry Univ, Jiangsu Coinnovat Ctr Efficient Proc & Utilizat F, Nanjing 210037, Peoples R China
2.Nanjing Forestry Univ, Int Innovat Ctr Forest Chem & Mat, Nanjing 210037, Peoples R China
3.Qilu Univ Technol, Shandong Acad Sci, State Key Lab Biobased Mat & Green Papermaking, Jinan 250353, Peoples R China
4.Nanjing IPE Inst Green Mfg Ind, Nanjing 211135, Peoples R China
5.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China
6.Univ New Brunswick, Dept Chem Engn, Fredericton, NB E3B 5A3, Canada
推荐引用方式
GB/T 7714
Dong, Maolin,Wu, Chen,Chen, Lidong,et al. Benzenesulfonic acid-based hydrotropic system for achieving lignocellulose separation and utilization under mild conditions[J]. BIORESOURCE TECHNOLOGY,2021,337:7.
APA Dong, Maolin.,Wu, Chen.,Chen, Lidong.,Zhou, Xuelian.,Yang, Weisheng.,...&Bian, Huiyang.(2021).Benzenesulfonic acid-based hydrotropic system for achieving lignocellulose separation and utilization under mild conditions.BIORESOURCE TECHNOLOGY,337,7.
MLA Dong, Maolin,et al."Benzenesulfonic acid-based hydrotropic system for achieving lignocellulose separation and utilization under mild conditions".BIORESOURCE TECHNOLOGY 337(2021):7.
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