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Assessing the contribution of atmospheric transport and tourism activities to the occurrence of perfluoroalkyl acids (PFAAs) in an Alpine Nature Reserve
Wang, Chenchen1,3; Lu, Yonglong1,3; Li, Qifeng2,4; Cao, Xianghui1,3; Zhang, Meng1,3; Zhou, Yunqiao1,3; Song, Shuai1; Wang, Pei1; Lu, Xiaotian5; Yvette, Baninla1,3
刊名SCIENCE OF THE TOTAL ENVIRONMENT
2019-12-20
卷号697页码:11
关键词Pfba Alpine Lake Snow Deposition Source Analysis
ISSN号0048-9697
DOI10.1016/j.scitotenv.2019.133851
英文摘要

Perfluoroalkyl acids (PFAAs) are ubiquitous in the global environment, even in remote regions. With increasing production and application of PFAAs in China, their distribution patterns have been widely reported, however with less attention to inland northwestern regions. Long-range transport and direct releases from local activities have been regarded as the main reasons for PFAAs distribution in such a remote area. To identify and quantify the contributions of different sources to PFAAs occurrences, an investigation was conducted in the Tianchi lake, nature reserve. A total of 20 water samples, 8 soil, 4 sediment and 10 fresh snow samples were collected and analyzed in 2015. The mean PFAAs concentrations were 3.38 ng L-1 in surface water, 1.06 ng g(-1) dw in soil, 0.53 ng g(-1) dw in sediment, and 3.31 ng L-1 in fresh snow, respectively. High levels of PFAAs were observed in surface water (15.41 ng L-1) from Western Tianchi pond and surface snow (14.24 ng L-1) from the site near a ski resort around Tianchi Lake indicating potential pollution by local human activities. The correlation between individual concentrations among water, soil and snow indicated the snow deposition as an important source. Although with limited sample size, principal component analysis associated with multiple linear regression (PCA-MLR) and positive matrix factorization (PMF) analyses have identified two major sources, which are characterized as tourism activities with dominance of perfluorooctanoic acid (PFOA) and long-range transport with abundant perfluorobutanoic acid (PFBA). Their contributions to total levels were 41% and 52%, respectively. These two sources contributed differently to the PFAAs presences in Tianchi and Western Tianchi Lakes. Source analysis indicates that the western Tianchi lake with a relatively small catchment was affected mainly by local activities. (C) 2019 Elsevier B.V. All rights reserved.

资助项目National Natural Science Foundation of China[41420104004] ; National Natural Science Foundation of China[71761147001] ; National Key Research and Development Program of China[2017YFC0505704] ; Key Project of the Chinese Academy of Sciences[KFZD-SW-322]
WOS关键词Fluorochemical Industrial Park ; Perfluorinated Alkyl Substances ; Polyfluoroalkyl Substances ; Perfluorooctane Sulfonate ; Fluorinated Alternatives ; Source Identification ; Source Apportionment ; Temporal Trends ; Coastal Region ; Drinking-water
WOS研究方向Environmental Sciences & Ecology
语种英语
出版者ELSEVIER
WOS记录号WOS:000499668600012
资助机构National Natural Science Foundation of China ; National Key Research and Development Program of China ; Key Project of the Chinese Academy of Sciences
内容类型期刊论文
源URL[http://ir.ipe.ac.cn/handle/122111/38414]  
专题中国科学院过程工程研究所
通讯作者Lu, Yonglong
作者单位1.Chinese Acad Sci, Res Ctr Ecoenvironm Sci, State Key Lab Urban & Reg Ecol, Beijing 100085, Peoples R China
2.Chinese Acad Sci, Innovat Acad Green Manufacture, Beijing 100190, Peoples R China
3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
4.Chinese Acad Sci, Inst Proc Engn, Beijing 100190, Peoples R China
5.Chinese Acad Sci, Inst Urban Environm, Key Lab Urban Environm & Hlth, 1799 Jimei Rd, Xiamen 361021, Fujian, Peoples R China
6.Chinese Acad Sci, Inst Soil Sci, Key Lab Soil Environm & Pollut Remediat, Nanjing 210008, Jiangsu, Peoples R China
推荐引用方式
GB/T 7714
Wang, Chenchen,Lu, Yonglong,Li, Qifeng,et al. Assessing the contribution of atmospheric transport and tourism activities to the occurrence of perfluoroalkyl acids (PFAAs) in an Alpine Nature Reserve[J]. SCIENCE OF THE TOTAL ENVIRONMENT,2019,697:11.
APA Wang, Chenchen.,Lu, Yonglong.,Li, Qifeng.,Cao, Xianghui.,Zhang, Meng.,...&Liu, Zhaoyang.(2019).Assessing the contribution of atmospheric transport and tourism activities to the occurrence of perfluoroalkyl acids (PFAAs) in an Alpine Nature Reserve.SCIENCE OF THE TOTAL ENVIRONMENT,697,11.
MLA Wang, Chenchen,et al."Assessing the contribution of atmospheric transport and tourism activities to the occurrence of perfluoroalkyl acids (PFAAs) in an Alpine Nature Reserve".SCIENCE OF THE TOTAL ENVIRONMENT 697(2019):11.
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