Dodecylamine assisted perovskite growth for high-performance perovskite solar cells with low defect density
He, Dingchao1,2; Yang, Zhiqian1,2; Li, Dufeng2; Niu, Yuanjuan1,2; Hu, Linhua2
刊名MATERIALS LETTERS
2022-02-15
卷号309
关键词Perovskite solar cell Mixed anti-solvent Crystal growth Defects
ISSN号0167-577X
DOI10.1016/j.matlet.2021.131365
通讯作者Hu, Linhua(lhhu@rntek.cas.cn)
英文摘要We correlated the concentration of alkylamine in the mixed anti-solvent with the growth process of the perovskite films and the defect passivation effect. The assisted crystal growth process based on "Ostwald ripening" was proposed. Benefiting from the assisted growth effect of dodecylamine on perovskite, the perovskite films have improved crystallinity, optimized interface, reduced defect concentration and suppressed nonradiative recombination of carriers. As a result, a power conversion efficiency of 21.67% was obtained for the devices based on mixed anti-solvent. And owing to the inherent hydrophobicity of the alkyl chains, the devices also have excellent humidity stability. This work provides a facile way to obtain high-quality perovskite films.
资助项目National Key R&D Program of China[2017YFE0133800] ; National Natural Science Foundation of China[51961165106] ; Anhui Provincial Natural Science Foundation[1908085QB52]
WOS关键词IODIDE
WOS研究方向Materials Science ; Physics
语种英语
出版者ELSEVIER
WOS记录号WOS:000736671800007
资助机构National Key R&D Program of China ; National Natural Science Foundation of China ; Anhui Provincial Natural Science Foundation
内容类型期刊论文
源URL[http://ir.hfcas.ac.cn:8080/handle/334002/127155]  
专题中国科学院合肥物质科学研究院
通讯作者Hu, Linhua
作者单位1.Univ Sci & Technol China, 96 Jinzhai Rd, Hefei 230026, Peoples R China
2.Chinese Acad Sci, Inst Solid State Phys, Key Lab Photovolta & Energy Conservat Mat, HFIPS, Hefei 230031, Peoples R China
推荐引用方式
GB/T 7714
He, Dingchao,Yang, Zhiqian,Li, Dufeng,et al. Dodecylamine assisted perovskite growth for high-performance perovskite solar cells with low defect density[J]. MATERIALS LETTERS,2022,309.
APA He, Dingchao,Yang, Zhiqian,Li, Dufeng,Niu, Yuanjuan,&Hu, Linhua.(2022).Dodecylamine assisted perovskite growth for high-performance perovskite solar cells with low defect density.MATERIALS LETTERS,309.
MLA He, Dingchao,et al."Dodecylamine assisted perovskite growth for high-performance perovskite solar cells with low defect density".MATERIALS LETTERS 309(2022).
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