Bifunctional Photoelectrode Driven by Charged Domain Walls in Ferroelectric Bi2WO6
Ullah, Rizwan; Pei, Minghui; Wu, Junsheng; Tian, Yu; Gu, Zhenao; Zhang, Qinghua; Song, Chuangye; Yang, Yuben; Ahmed, Munir; Zeb, Johar
刊名ACS APPLIED ENERGY MATERIALS
2020-05-26
卷号3期号:5页码:4149-4154
关键词bifunctional photocatalysts photoelectrochemical water splitting Aurivillius perovskite Bi2WO6 ferroelectric domain charged domain wall
ISSN号2574-0962
英文摘要Photoelectrochemical technology provides a promising way to solve the emerging energy crisis, yet it still faces obstacles like weak charge transfer and separation of traditional photoelectrodes. Here, by using single crystalline epitaxial ferroelectric Bi2WO6 thin films, a bifunctional photoelectrode for photoelectrochemical water splitting is demonstrated, which originates from the in-plane ferroelectricity and charged domain walls. The optimized anodic (cathodic) photocurrent density is 0.175 (0.240) mA cm(-2) at 1.23 V (0 V) vs RHE in Na2SO4 (pH = 7) electrolyte solution. Manipulations of the in-plane polarization and charged domain walls provide an alternative catalyzing strategy toward efficient and controllable photoelectrochemical water splitting.
内容类型期刊论文
源URL[http://ir.rcees.ac.cn/handle/311016/45242]  
专题生态环境研究中心_中国科学院饮用水科学与技术重点实验室
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GB/T 7714
Ullah, Rizwan,Pei, Minghui,Wu, Junsheng,et al. Bifunctional Photoelectrode Driven by Charged Domain Walls in Ferroelectric Bi2WO6[J]. ACS APPLIED ENERGY MATERIALS,2020,3(5):4149-4154.
APA Ullah, Rizwan.,Pei, Minghui.,Wu, Junsheng.,Tian, Yu.,Gu, Zhenao.,...&Zhang, Jinxing.(2020).Bifunctional Photoelectrode Driven by Charged Domain Walls in Ferroelectric Bi2WO6.ACS APPLIED ENERGY MATERIALS,3(5),4149-4154.
MLA Ullah, Rizwan,et al."Bifunctional Photoelectrode Driven by Charged Domain Walls in Ferroelectric Bi2WO6".ACS APPLIED ENERGY MATERIALS 3.5(2020):4149-4154.
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