Distributions and sources of n-alkanes in PM2.5 at urban, industrial and coastal sites in Tianjin, China | |
Li Weifang3; Peng Yue1; Bai Zhipeng3 | |
刊名 | JOURNAL OF ENVIRONMENTAL SCIENCES |
2010 | |
卷号 | 22期号:10页码:1551-1557 |
关键词 | POLYCYCLIC AROMATIC-HYDROCARBONS AIR-POLLUTION SOURCES ORGANIC AEROSOL PARTICULATE MATTER MOLECULAR COMPOSITION SOURCE APPORTIONMENT TRACERS PHASE ATMOSPHERE COMPONENTS PM2.5 n-alkanes distribution pattern CPIs plant wax |
ISSN号 | 1001-0742 |
其他题名 | Distributions and sources of n-alkanes in PM 2.5 at urban, industrial and coastal sites in Tianjin, China |
英文摘要 | Aliphatic hydrocarbons (n-alkanes) associated with fine particulate matter were determined in the ambient air of urban, industrial and coastal areas in Tianjin, China, where intensive coal burning for industrial and domestic purpose takes place. n-Alkane homologues from C12 to C35 were quantifiable in all samples with C20-C31 being the most abundant species. Average concentrations of the total n-alkanes were 148.7, 250.1 and 842.0 ng/m(3) in July, April and January, respectively. Seasonal variations were mainly attributed to ambient temperature changes and coal combustion for residential heating. Among the three studied areas, the highest levels of n-alkanes were observed in the industrial complex in winter and spring, but in summer the coastal alkane concentration moved up to the highest. A mono-modal distribution for n-alkanes was observed in spring and summer with odd carbon number predominance and a maximum centered at C27-C31, suggesting the release of plant wax into the atmosphere. The bimodal distribution with maxima at C22 and C26 observed in winter indicated a substantial influence of fossil fuel sources. All the CPIs (CPI1, CPI2, CPI3) values, varying between 0.64 and 1.97, indicated the influence of anthropogenic emissions on fine organic aerosols. The estimated contributions of plant wax to total n-alkanes were on average of 12.9%, 19.1% and 26.1% for winter, spring and summer, respectively. |
资助项目 | [Commonweal Project of National Environment Protection] ; [National Basic Research Program (973) of China] |
语种 | 英语 |
CSCD记录号 | CSCD:4036700 |
内容类型 | 期刊论文 |
源URL | [http://ir.imr.ac.cn/handle/321006/154228] |
专题 | 金属研究所_中国科学院金属研究所 |
作者单位 | 1.中国科学院金属研究所 2.Tianjin Acad Environm Protect Science, Tianjin 300191, Peoples R China 3.南开大学 |
推荐引用方式 GB/T 7714 | Li Weifang,Peng Yue,Bai Zhipeng. Distributions and sources of n-alkanes in PM2.5 at urban, industrial and coastal sites in Tianjin, China[J]. JOURNAL OF ENVIRONMENTAL SCIENCES,2010,22(10):1551-1557. |
APA | Li Weifang,Peng Yue,&Bai Zhipeng.(2010).Distributions and sources of n-alkanes in PM2.5 at urban, industrial and coastal sites in Tianjin, China.JOURNAL OF ENVIRONMENTAL SCIENCES,22(10),1551-1557. |
MLA | Li Weifang,et al."Distributions and sources of n-alkanes in PM2.5 at urban, industrial and coastal sites in Tianjin, China".JOURNAL OF ENVIRONMENTAL SCIENCES 22.10(2010):1551-1557. |
个性服务 |
查看访问统计 |
相关权益政策 |
暂无数据 |
收藏/分享 |
除非特别说明,本系统中所有内容都受版权保护,并保留所有权利。
修改评论