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A Double Support Layer for Facile Clean Transfer of Two-Dimensional Materials for High-Performance Electronic and Optoelectronic Devices
Zhang, Dingdong1,2; Du, Jinhong1,2; Hong, Yi-Lun1,2; Zhang, Weimin1,2; Wang, Xiao3; Jin, Hui3; Burn, Paul L.3; Yu, Junsheng4; Chen, Maolin1,2; Sun, Dong-Min1,2
刊名ACS NANO
2019-05-01
卷号13期号:5页码:5513-5522
关键词rosin graphene 2D materials clean transfer optoelectronic devices
ISSN号1936-0851
DOI10.1021/acsnano.9b00330
通讯作者Ren, Wencai(wcren@imr.ac.cn)
英文摘要Clean transfer of two-dimensional (2D) materials grown by chemical vapor deposition is critical for their application in electronics and optoelectronics. Although rosin can be used as a support layer for the clean transfer of graphene grown on Cu, it has not been usable for the transfer of 2D materials grown on noble metals or for large-area transfer. Here, we report a poly(methyl methacrylate) (PMMA)/rosin double support layer that enables facile ultraclean transfer of large-area 2D materials glown on different metals. The bottom rosin layer ensures clean transfer, whereas the top PMMA layer not only screens the rosin from the transfer conditions but also improves the strength of the transfer layer to make the transfer easier and more robust. We demonstrate the transfer of monolayer WSe, and WS2 single crystals grown on Au as well as large-area graphene films grown on Cu. As a result of the clean surface, the transferred WSe2 retains the intrinsic optical properties of the as-grown sample. Moreover, it does not require annealing to form good ohmic contacts with metal electrodes, enabling highperformance field effect transistors with mobility and ON/OFF ratio,--10 times higher than those made by PMMAtransferred WSe2. The ultraclean graphene film is found to be a good anode for flexible organic photovoltaic cells with a high power conversion efficiency of,-6.4% achieved.
资助项目Ministry of Science and Technology of China[2016YFA0200101] ; National Science Foundation of China[51572265] ; National Science Foundation of China[51861135201] ; National Science Foundation of China[51325205] ; National Science Foundation of China[51290273] ; National Science Foundation of China[51521091] ; Chinese Academy of Sciences[KGZD-EW-303-1] ; Chinese Academy of Sciences[KGZD-EW-303-3] ; Postdoctoral Science Foundation of China[2018M630309] ; Strategic Priority Research Program of Chinese Academy of Sciences[XDB30000000] ; Australian Research Council[FL160100067] ; Australian Government through the Australian Renewable Energy Agency (ARENA) Australian Centre for Advanced Photovoltaics
WOS研究方向Chemistry ; Science & Technology - Other Topics ; Materials Science
语种英语
出版者AMER CHEMICAL SOC
WOS记录号WOS:000469886300057
资助机构Ministry of Science and Technology of China ; National Science Foundation of China ; Chinese Academy of Sciences ; Postdoctoral Science Foundation of China ; Strategic Priority Research Program of Chinese Academy of Sciences ; Australian Research Council ; Australian Government through the Australian Renewable Energy Agency (ARENA) Australian Centre for Advanced Photovoltaics
内容类型期刊论文
源URL[http://ir.imr.ac.cn/handle/321006/133852]  
专题金属研究所_中国科学院金属研究所
通讯作者Ren, Wencai
作者单位1.Chinese Acad Sci, Shenyang Natl Lab Mat Sci, Inst Met Res, 72 Wenhua Rd, Shenyang 110016, Liaoning, Peoples R China
2.Univ Sci & Technol China, Sch Mat Sci & Engn, 72 Wenhua Rd, Shenyang 110016, Liaoning, Peoples R China
3.Univ Queensland, Sch Chem & Mol Biosci, Ctr Organ Photon & Elect, Brisbane, Qld 4072, Australia
4.UESTC, Sch Optoelect Sci & Engn, State Key Lab Elect Thin Films & Integrated Devic, Chengdu 610054, Sichuan, Peoples R China
5.Chinese Acad Sci, Shenyang Inst Automat, 114 Nanta St, Shenyang 110016, Liaoning, Peoples R China
6.Tsinghua Univ, Tsinghua Berkeley Shenzhen Inst, Shenzhen Geim Graphene Ctr, 1001 Xueyuan Rd, Shenzhen 518055, Peoples R China
推荐引用方式
GB/T 7714
Zhang, Dingdong,Du, Jinhong,Hong, Yi-Lun,et al. A Double Support Layer for Facile Clean Transfer of Two-Dimensional Materials for High-Performance Electronic and Optoelectronic Devices[J]. ACS NANO,2019,13(5):5513-5522.
APA Zhang, Dingdong.,Du, Jinhong.,Hong, Yi-Lun.,Zhang, Weimin.,Wang, Xiao.,...&Ren, Wencai.(2019).A Double Support Layer for Facile Clean Transfer of Two-Dimensional Materials for High-Performance Electronic and Optoelectronic Devices.ACS NANO,13(5),5513-5522.
MLA Zhang, Dingdong,et al."A Double Support Layer for Facile Clean Transfer of Two-Dimensional Materials for High-Performance Electronic and Optoelectronic Devices".ACS NANO 13.5(2019):5513-5522.
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