The effect of carbon support on the oxygen reduction activity and durability of single-atom iron catalysts

doi:10.1557/mrc.2018.174

CORC > 金属研究所 > 中国科学院金属研究所

	The effect of carbon support on the oxygen reduction activity and durability of single-atom iron catalysts
	Li, Jin-Cheng 1,2; Tang, Dai-Ming 1; Hou, Peng-Xiang 1; Li, Guo-Xian 1; Cheng, Min 1; Liu, Chang 1; Cheng, Hui-Ming 1,3
刊名	MRS COMMUNICATIONS
	2018-09-01
卷号	8 期号:3 页码:1158-1166
ISSN号	2159-6859
DOI	10.1557/mrc.2018.174
通讯作者	Hou, Peng-Xiang(pxhou@imr.ac.cn) ; Liu, Chang(cliu@imr.ac.cn)
英文摘要	Owing to lack of a definitive correlation between carbon supports and catalytic activity of single-atom Fe-active sites, rational design and preparation of single-atom Fe catalysts have so far been elusive. Herein we designed and prepared one-dimensional core-shell nanostructured single-atom Fe catalysts, in which carbon nanofibers and carbon nanotubes with different crystallinities and electrical conductivities were used as supports to host single-atom Fe-active sites. It was found that the carbon supports with higher electrical conductivity accelerate charge transfer and enhance the oxygen reduction reaction (ORR) activity of single-atom Fe-active sites as well as the ORR durability of the final catalyst.
资助项目	Ministry of Science and Technology of China[2016YFA0200102] ; National Natural Science Foundation of China[51625203] ; National Natural Science Foundation of China[51532008] ; National Natural Science Foundation of China[51521091] ; National Natural Science Foundation of China[51772303] ; National Natural Science Foundation of China[51572264] ; Chinese Academy of Sciences[KGZD-EW-T06] ; CAS/SAFEA International Partnership Program for Creative Research Teams ; Liaoning BaiQianWan Talents Program
WOS研究方向	Materials Science
语种	英语
出版者	CAMBRIDGE UNIV PRESS
WOS记录号	WOS:000448887900067
资助机构	Ministry of Science and Technology of China ; National Natural Science Foundation of China ; Chinese Academy of Sciences ; CAS/SAFEA International Partnership Program for Creative Research Teams ; Liaoning BaiQianWan Talents Program
内容类型	期刊论文
源URL	[http://ir.imr.ac.cn/handle/321006/130118]
专题	金属研究所_中国科学院金属研究所
通讯作者	Hou, Peng-Xiang; Liu, Chang
作者单位	1.Chinese Acad Sci, Shenyang Natl Lab Mat Sci, Inst Met Res, Shenyang 110016, Liaoning, Peoples R China 2.Hong Kong Univ Sci & Technol, Fok Ying Tung Res Inst, Guangzhou 511458, Guangdong, Peoples R China 3.Tsinghua Univ, Tsinghua Berkeley Shenzhen Inst, Shenzhen 5108055, Peoples R China
推荐引用方式 GB/T 7714	Li, Jin-Cheng,Tang, Dai-Ming,Hou, Peng-Xiang,et al. The effect of carbon support on the oxygen reduction activity and durability of single-atom iron catalysts[J]. MRS COMMUNICATIONS,2018,8(3):1158-1166.
APA	Li, Jin-Cheng.,Tang, Dai-Ming.,Hou, Peng-Xiang.,Li, Guo-Xian.,Cheng, Min.,...&Cheng, Hui-Ming.(2018).The effect of carbon support on the oxygen reduction activity and durability of single-atom iron catalysts.MRS COMMUNICATIONS,8(3),1158-1166.
MLA	Li, Jin-Cheng,et al."The effect of carbon support on the oxygen reduction activity and durability of single-atom iron catalysts".MRS COMMUNICATIONS 8.3(2018):1158-1166.