Dual response mimetic enzyme of novel Co4S3/Co3O4 composite nanotube for antibacterial application | |
Wang, Jin1,2,5,6; Wang, Yi1,2,5; Zhang, Dun1,2,5; Xu, Chaojie3,6; Xing, Ronge2,3,4 | |
刊名 | JOURNAL OF HAZARDOUS MATERIALS |
2020-06-15 | |
卷号 | 392页码:11 |
关键词 | Co4S3/Co3O4 nanotubes Kirkendall effect Oxidase and peroxidase Broad spectrum sterilization Biocompatibility |
ISSN号 | 0304-3894 |
DOI | 10.1016/j.jhazmat.2020.122278 |
通讯作者 | Wang, Yi(wangyi@qdio.ac.cn) ; Zhang, Dun(zhangdun@qdio.ac.cn) |
英文摘要 | Novel Co4S3/Co3O4 composite nanotubes were first time successfully synthesized through the control of Na2S treatment of Co(CO3)(0.35)Cl-0.20(OH)(1.10) precursor and testified to having both oxidase-like and peroxidase-like catalytic activities. Through nanoscale Kirkendall effect, acicular precursor was vulcanized to form Co4S3/Co3O4 nanotubes (NTs). Co4S3/Co3O4 NTs exhibit great properties such as smaller K-m and higher V(max )than natural horseradish peroxidase, favorable selectivity and ideal stability. Co4S3/Co3O4 NTs with promising biocompatibility can realize spectral sterilization towards Escherichia coll. and Staphylococcus sciuri in the presence of low level H2O2. It turned to be that superoxide anion radical catalyzed by Co4S3/Co3O4 NTs not only oxidizes 3, 3', 5, 5'-tetramethylbenzidine in the catalytic process but also eliminates gram-bacteria during sterilization. The successful synthesis of biofunctional Co4S3/Co3O4 NTs can serve as significant applications of new energy and environmental catalysis. |
资助项目 | Natured Science Foundation of China[41776090] ; Natured Science Foundation of China[41976032] ; National Key Research and Development Program of China[2016YFC1400605] ; Highend users Program of Kexue[KEXUE2019GZ01] ; Key Research and Development Program of Shandong Province[2018GHY115038] ; AoShan Talent Program - Qingdao National Laboratory for Marine Science and Technology |
WOS研究方向 | Engineering ; Environmental Sciences & Ecology |
语种 | 英语 |
出版者 | ELSEVIER |
WOS记录号 | WOS:000527016900030 |
内容类型 | 期刊论文 |
源URL | [http://ir.qdio.ac.cn/handle/337002/167280] |
专题 | 海洋研究所_海洋腐蚀与防护研究发展中心 |
通讯作者 | Wang, Yi; Zhang, Dun |
作者单位 | 1.Pilot Natl Lab Marine Sci & Technol, Open Studio Marine Corros & Protect, 1 Wenhai Rd, Qingdao 266237, Peoples R China 2.Chinese Acad Sci, Ctr Ocean Mega Sci, 7 Nanhai Rd, Qingdao 266071, Peoples R China 3.Chinese Acad Sci, Inst Oceanol, CAS Key Lab Expt Marine Biol, 7 Nanhai Rd, Qingdao 266071, Peoples R China 4.Pilot Natl Lab Marine Sci & Technol, Lab Marine Drugs & Bioprod, 1 Wenhai Rd, Qingdao 266237, Peoples R China 5.Chinese Acad Sci, Inst Oceanol, CAS Key Lab Marine Environm Corros & Biofouling, 7 Nanhai Rd, Qingdao 266071, Peoples R China 6.Univ Chinese Acad Sci, 19 Jia Yuquan Rd, Beijing 100039, Peoples R China |
推荐引用方式 GB/T 7714 | Wang, Jin,Wang, Yi,Zhang, Dun,et al. Dual response mimetic enzyme of novel Co4S3/Co3O4 composite nanotube for antibacterial application[J]. JOURNAL OF HAZARDOUS MATERIALS,2020,392:11. |
APA | Wang, Jin,Wang, Yi,Zhang, Dun,Xu, Chaojie,&Xing, Ronge.(2020).Dual response mimetic enzyme of novel Co4S3/Co3O4 composite nanotube for antibacterial application.JOURNAL OF HAZARDOUS MATERIALS,392,11. |
MLA | Wang, Jin,et al."Dual response mimetic enzyme of novel Co4S3/Co3O4 composite nanotube for antibacterial application".JOURNAL OF HAZARDOUS MATERIALS 392(2020):11. |
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