Dual response mimetic enzyme of novel Co4S3/Co3O4 composite nanotube for antibacterial application
Wang, Jin1,2,5,6; Wang, Yi1,2,5; Zhang, Dun1,2,5; Xu, Chaojie3,6; Xing, Ronge2,3,4
刊名JOURNAL OF HAZARDOUS MATERIALS
2020-06-15
卷号392页码:11
关键词Co4S3/Co3O4 nanotubes Kirkendall effect Oxidase and peroxidase Broad spectrum sterilization Biocompatibility
ISSN号0304-3894
DOI10.1016/j.jhazmat.2020.122278
通讯作者Wang, Yi(wangyi@qdio.ac.cn) ; Zhang, Dun(zhangdun@qdio.ac.cn)
英文摘要Novel Co4S3/Co3O4 composite nanotubes were first time successfully synthesized through the control of Na2S treatment of Co(CO3)(0.35)Cl-0.20(OH)(1.10) precursor and testified to having both oxidase-like and peroxidase-like catalytic activities. Through nanoscale Kirkendall effect, acicular precursor was vulcanized to form Co4S3/Co3O4 nanotubes (NTs). Co4S3/Co3O4 NTs exhibit great properties such as smaller K-m and higher V(max )than natural horseradish peroxidase, favorable selectivity and ideal stability. Co4S3/Co3O4 NTs with promising biocompatibility can realize spectral sterilization towards Escherichia coll. and Staphylococcus sciuri in the presence of low level H2O2. It turned to be that superoxide anion radical catalyzed by Co4S3/Co3O4 NTs not only oxidizes 3, 3', 5, 5'-tetramethylbenzidine in the catalytic process but also eliminates gram-bacteria during sterilization. The successful synthesis of biofunctional Co4S3/Co3O4 NTs can serve as significant applications of new energy and environmental catalysis.
资助项目Natured Science Foundation of China[41776090] ; Natured Science Foundation of China[41976032] ; National Key Research and Development Program of China[2016YFC1400605] ; Highend users Program of Kexue[KEXUE2019GZ01] ; Key Research and Development Program of Shandong Province[2018GHY115038] ; AoShan Talent Program - Qingdao National Laboratory for Marine Science and Technology
WOS研究方向Engineering ; Environmental Sciences & Ecology
语种英语
出版者ELSEVIER
WOS记录号WOS:000527016900030
内容类型期刊论文
源URL[http://ir.qdio.ac.cn/handle/337002/167280]  
专题海洋研究所_海洋腐蚀与防护研究发展中心
通讯作者Wang, Yi; Zhang, Dun
作者单位1.Pilot Natl Lab Marine Sci & Technol, Open Studio Marine Corros & Protect, 1 Wenhai Rd, Qingdao 266237, Peoples R China
2.Chinese Acad Sci, Ctr Ocean Mega Sci, 7 Nanhai Rd, Qingdao 266071, Peoples R China
3.Chinese Acad Sci, Inst Oceanol, CAS Key Lab Expt Marine Biol, 7 Nanhai Rd, Qingdao 266071, Peoples R China
4.Pilot Natl Lab Marine Sci & Technol, Lab Marine Drugs & Bioprod, 1 Wenhai Rd, Qingdao 266237, Peoples R China
5.Chinese Acad Sci, Inst Oceanol, CAS Key Lab Marine Environm Corros & Biofouling, 7 Nanhai Rd, Qingdao 266071, Peoples R China
6.Univ Chinese Acad Sci, 19 Jia Yuquan Rd, Beijing 100039, Peoples R China
推荐引用方式
GB/T 7714
Wang, Jin,Wang, Yi,Zhang, Dun,et al. Dual response mimetic enzyme of novel Co4S3/Co3O4 composite nanotube for antibacterial application[J]. JOURNAL OF HAZARDOUS MATERIALS,2020,392:11.
APA Wang, Jin,Wang, Yi,Zhang, Dun,Xu, Chaojie,&Xing, Ronge.(2020).Dual response mimetic enzyme of novel Co4S3/Co3O4 composite nanotube for antibacterial application.JOURNAL OF HAZARDOUS MATERIALS,392,11.
MLA Wang, Jin,et al."Dual response mimetic enzyme of novel Co4S3/Co3O4 composite nanotube for antibacterial application".JOURNAL OF HAZARDOUS MATERIALS 392(2020):11.
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