AcOH-mediated aerobic oxidative synthesis of 2-thioalkylbenzothiazoles via a three-component reaction | |
Li, Xiaowei2,3,4; Li, Yuxiu1; Liu, Ruihua1; Wang, Zemin1; Li, Xiangqian1; Shi, Dayong1,3,4 | |
刊名 | TETRAHEDRON LETTERS |
2020-06-25 | |
卷号 | 61期号:26页码:5 |
关键词 | 2-Thioalkylbenzothiazoles Metal-free Aerobic oxidation Multicomponent reaction |
ISSN号 | 0040-4039 |
DOI | 10.1016/j.tetlet.2020.152054 |
通讯作者 | Shi, Dayong(shidayong@sdu.edu.cn) |
英文摘要 | An AcOH-mediated three-component reaction of 2-aminothiophenols, alpha,beta-unsaturated aldehydes, and thiophenols to prepare the high value-added 2-thioalkylbenzothiazoles was developed. The reaction was conducted under metal-free conditions, where oxygen served as the terminal oxidant. In addition, this strategy is tolerant of kinds of functional groups, providing efficient access to a variety of functionalized benzothiazole derivatives in moderate to good yields. What's more, this reaction has complete regioslectivity and provides a powerful method for building complex molecules. (C) 2020 Elsevier Ltd. All rights reserved. |
资助项目 | Shandong Provincial Natural Science Foundation for Distinguished Young Scholars[JQ201722] ; Taishan scholar Youth Project of Shandong province ; Qingdao Marine Biomedical Science and Technology Innovation Center Project[2017-CXZX01-1-1] ; Qingdao Marine Biomedical Science and Technology Innovation Center Project[2017-CXZX01-3-9] ; NSFC-Shandong Joint Fund[U1706213] ; National Natural Science Foundation of China[81803344] ; China Postdoctoral Science Foundation[2019M662374] ; China Postdoctoral Science Foundation[2019M662377] ; China Postdoctoral Science Foundation[2019M662378] ; National Program for Support of Top-notch Young Professionals ; Key research and development plan (soft science) project of Shandong province[2019RKE27018] |
WOS研究方向 | Chemistry |
语种 | 英语 |
出版者 | PERGAMON-ELSEVIER SCIENCE LTD |
WOS记录号 | WOS:000540277100014 |
内容类型 | 期刊论文 |
源URL | [http://ir.qdio.ac.cn/handle/337002/167672] |
专题 | 海洋研究所_实验海洋生物学重点实验室 |
通讯作者 | Shi, Dayong |
作者单位 | 1.Shandong Univ, State Key Lab Microbial Technol, 72 Binhai Rd, Qingdao 266237, Peoples R China 2.Chinese Acad Sci, Inst Oceanol, Key Lab Expt Marine Biol, 7 Nanhai Rd, Qingdao 266071, Shandong, Peoples R China 3.Qingdao Natl Lab Marine Sci & Technol, Lab Marine Drugs & Bioprod, Qingdao 266000, Peoples R China 4.Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
推荐引用方式 GB/T 7714 | Li, Xiaowei,Li, Yuxiu,Liu, Ruihua,et al. AcOH-mediated aerobic oxidative synthesis of 2-thioalkylbenzothiazoles via a three-component reaction[J]. TETRAHEDRON LETTERS,2020,61(26):5. |
APA | Li, Xiaowei,Li, Yuxiu,Liu, Ruihua,Wang, Zemin,Li, Xiangqian,&Shi, Dayong.(2020).AcOH-mediated aerobic oxidative synthesis of 2-thioalkylbenzothiazoles via a three-component reaction.TETRAHEDRON LETTERS,61(26),5. |
MLA | Li, Xiaowei,et al."AcOH-mediated aerobic oxidative synthesis of 2-thioalkylbenzothiazoles via a three-component reaction".TETRAHEDRON LETTERS 61.26(2020):5. |
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