First measurement of atmospheric mercury species in Qomolangma Natural Nature Preserve, Tibetan Plateau, and evidence oftransboundary pollutant invasion
Huiming Lin;  Yindong Tong;  Xiufeng Yin;  Qianggong Zhang;  Hui Zhang;  Haoran Zhang;  Long Chen;  Shichang Kang;  Wei Zhang;  James Schauer;  Benjamin de Foy;  Xiaoge Bu;  Xuejun Wang
刊名Atmospheric Chemistry and Physics 19(2), pp.
2019
卷号19期号:2页码:1373-1391
英文摘要

Located in the world's “third pole” and a remote region connecting the Indian plate and the Eurasian plate, Qomolangma National Nature Preserve (QNNP) is an ideal region to study the long-range transport of atmospheric pollutants. In this study, gaseous elemental mercury (GEM), gaseous oxidized mercury (GOM) and particle-bound mercury (PBM) were continuously measured during the Indian monsoon transition period in QNNP. A slight increase in the GEM concentration was observed from the period preceding the Indian summer monsoon (1.31±0.42 ng m−3) to the Indian summer monsoon period (1.44±0.36 ng m−3), while significant decreases were observed in the GOM and PBM concentrations, with concentrations decreasing from 35.2±18.6 to 19.3±10.9 pg m−3 (p< 0.001) for GOM and from 30.5±12.5 to 24.9±19.8 pg m−3 (p< 0.001) for PBM. A unique daily pattern was observed in QNNP with respect to the GEM concentration, with a peak value before sunrise and a low value at noon. Relative to the (low) GEM concentrations, GOM concentrations (with a mean value of 21.4±13.4 pg m−3n=1239) in this region were relatively high compared with the measured values in some other regions of China. A cluster analysis indicated that the air masses transported to QNNP changed significantly at different stages of the monsoon, and the major potential mercury (Hg) sources shifted from northern India and western Nepal to eastern Nepal and Bangladesh. As there is a large area covered in glaciers in QNNP, local glacier winds could increase the transboundary transport of pollutants and transport polluted air masses to the Tibetan Plateau. The atmospheric Hg concentration in QNNP in the Indian summer monsoon period was influenced by transboundary Hg flows. This highlights the need for a more specific identification of Hg sources impacting QNNP and underscores the importance of international cooperation regarding global Hg controls.

语种英语
内容类型期刊论文
源URL[http://ir.gyig.ac.cn/handle/42920512-1/10916]  
专题地球化学研究所_环境地球化学国家重点实验室
作者单位1.University of Chinese Academy of Sciences, Beijing, 100039, China
2.MOE Laboratory of Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing, 100871, China
3.School of Environmental Science and Engineering, Tianjin University, Tianjin, 300072, China
4.State Key Laboratory of Cryospheric Science, Northwest Institute of Eco-Environment and Resources, Chinese Academy of Sciences, Lanzhou, 730000, China
5.Department of Earth and Atmospheric Sciences, Saint Louis University, Saint Louis, MO 63108, USA
6.Key Laboratory of Tibetan Environment Changes and Land Surface Processes, Institute of Tibetan Plateau Research, Chinese Academy of Sciences, Beijing, 100101, China
7.CAS Center for Excellence in Tibetan Plateau Earth Sciences, Beijing, 100085, China
8.State Key Laboratory of Environmental Geochemistry, Institute of Geochemistry, Chinese Academy of Sciences, Guiyang, 550002, China
9.School of Geographic Sciences, East China Normal University, Shanghai, 200241, China
10.School of Environment and Natural Resources, Renmin University of China, Beijing, 100872, China
推荐引用方式
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Huiming Lin;Yindong Tong;Xiufeng Yin;Qianggong Zhang;Hui Zhang;Haoran Zhang;Long Chen;Shichang Kang;Wei Zhang;James Schauer;Benjamin de Foy;Xiaoge Bu;Xuejun Wang. First measurement of atmospheric mercury species in Qomolangma Natural Nature Preserve, Tibetan Plateau, and evidence oftransboundary pollutant invasion[J]. Atmospheric Chemistry and Physics 19(2), pp.,2019,19(2):1373-1391.
APA Huiming Lin;Yindong Tong;Xiufeng Yin;Qianggong Zhang;Hui Zhang;Haoran Zhang;Long Chen;Shichang Kang;Wei Zhang;James Schauer;Benjamin de Foy;Xiaoge Bu;Xuejun Wang.(2019).First measurement of atmospheric mercury species in Qomolangma Natural Nature Preserve, Tibetan Plateau, and evidence oftransboundary pollutant invasion.Atmospheric Chemistry and Physics 19(2), pp.,19(2),1373-1391.
MLA Huiming Lin;Yindong Tong;Xiufeng Yin;Qianggong Zhang;Hui Zhang;Haoran Zhang;Long Chen;Shichang Kang;Wei Zhang;James Schauer;Benjamin de Foy;Xiaoge Bu;Xuejun Wang."First measurement of atmospheric mercury species in Qomolangma Natural Nature Preserve, Tibetan Plateau, and evidence oftransboundary pollutant invasion".Atmospheric Chemistry and Physics 19(2), pp. 19.2(2019):1373-1391.
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