Electric field controllable high-spin SrRuO3 driven by a solid ionic junction
Lu, Jingdi; Si, Liang; Yao, Xiefei; Tian, Chengfeng; Wang, Jing; Zhang, Qinghua; Lai, Zhengxun; Malik, Iftikhar Ahmed; Liu, Xin; Jiang, Peiheng
刊名PHYSICAL REVIEW B
2020
卷号101期号:21
关键词MAGNETIC-PROPERTIES SEMICONDUCTORS FERROMAGNETISM SPECTROSCOPY OXIDE
DOI10.1103/PhysRevB.101.214401
英文摘要Controlling magnetism and spin structures in strongly correlated systems by using electric fields is of fundamental importance but challenging. Here, a high-spin ruthenate phase is achieved via a solid ionic chemical junction at the SrRuO3/SrTiO3 interface with distinct formation energies and diffusion barriers of oxygen vacancies, an analog to electronic band alignment in the semiconductor heterojunction. Oxygen vacancies trapped within this interfacial SrRuO3 reconstruct the Ru-4d electronic structure and orbital occupancy, leading to an enhanced magnetic moment. Furthermore, this emergent interfacial magnetic phase can be switched reversibly by electric-field-rectifying oxygen migration in a solid-state ionic gating device, providing a framework for the atomic design of functionalities in strongly correlated oxides using a method of solid chemistry.
学科主题Materials Science ; Physics
内容类型期刊论文
源URL[http://ir.nimte.ac.cn/handle/174433/20765]  
专题2020专题
作者单位1.Zhong, ZC (corresponding author), Chinese Acad Sci, NIMTE, Key Lab Magnet Mat & Devices, Ningbo 315201, Peoples R China.
2.Zhong, ZC (corresponding author), Chinese Acad Sci, NIMTE, Zhejiang Prov Key Lab Magnet Mat & Applicat Techn, Ningbo 315201, Peoples R China.
推荐引用方式
GB/T 7714
Lu, Jingdi,Si, Liang,Yao, Xiefei,et al. Electric field controllable high-spin SrRuO3 driven by a solid ionic junction[J]. PHYSICAL REVIEW B,2020,101(21).
APA Lu, Jingdi.,Si, Liang.,Yao, Xiefei.,Tian, Chengfeng.,Wang, Jing.,...&Zhang, Jinxing.(2020).Electric field controllable high-spin SrRuO3 driven by a solid ionic junction.PHYSICAL REVIEW B,101(21).
MLA Lu, Jingdi,et al."Electric field controllable high-spin SrRuO3 driven by a solid ionic junction".PHYSICAL REVIEW B 101.21(2020).
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