Vapor-phase assisted hydrothermal carbon from sucrose and its application in acid catalysis | |
Zhong, R.2; Liao, Y.2; Shu, R.1; Ma, L.1; Sels, B. F.2 | |
刊名 | GREEN CHEMISTRY |
2018-03-21 | |
卷号 | 20期号:6页码:1345-1353 |
ISSN号 | 1463-9262 |
DOI | 10.1039/c7gc02236k |
通讯作者 | Sels, B. F.(bert.sels@kuleuven.be) |
英文摘要 | A novel and practical synthesis method for carbonaceous materials was proposed by the vapor-phase hydrothermal treatment of sucrose at a mild 200 degrees C temperature. The resultant carbon possesses a 52 m(2) g(-1) specific surface area and 0.18 cm(3) g(-1) total pore volume - values that are substantially higher than those of conventional hydrothermally treated sugar solutions. The functionalization of the porous carbon with -SO3H led to acidic materials with high catalytic activity and selectivity towards, e.g., the sylvan condensation with furfural. |
资助项目 | National Natural Science Foundation of China[51536009] ; Chinese Scholarship Council[201404910467] ; Chinese Scholarship Council[201206210307] |
WOS关键词 | MESOPOROUS CARBONS ; ENERGY-STORAGE ; SOLID ACID ; BIOMASS ; CONVERSION ; CARBONIZATION ; FRUCTOSE ; 2-METHYLFURAN ; SPECTROSCOPY ; ACTIVATION |
WOS研究方向 | Chemistry ; Science & Technology - Other Topics |
语种 | 英语 |
出版者 | ROYAL SOC CHEMISTRY |
WOS记录号 | WOS:000428088400022 |
资助机构 | National Natural Science Foundation of China ; Chinese Scholarship Council |
内容类型 | 期刊论文 |
源URL | [http://ir.giec.ac.cn/handle/344007/23287] |
专题 | 中国科学院广州能源研究所 |
通讯作者 | Sels, B. F. |
作者单位 | 1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy, Guangzhou 510640, Guangdong, Peoples R China 2.Katholieke Univ Leuven, Ctr Surface Sci & Catalysis, Corelab, Celestijnenlaan 200F, B-3001 Heverlee, Belgium |
推荐引用方式 GB/T 7714 | Zhong, R.,Liao, Y.,Shu, R.,et al. Vapor-phase assisted hydrothermal carbon from sucrose and its application in acid catalysis[J]. GREEN CHEMISTRY,2018,20(6):1345-1353. |
APA | Zhong, R.,Liao, Y.,Shu, R.,Ma, L.,&Sels, B. F..(2018).Vapor-phase assisted hydrothermal carbon from sucrose and its application in acid catalysis.GREEN CHEMISTRY,20(6),1345-1353. |
MLA | Zhong, R.,et al."Vapor-phase assisted hydrothermal carbon from sucrose and its application in acid catalysis".GREEN CHEMISTRY 20.6(2018):1345-1353. |
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