Activation strategies of water-splitting electrocatalysts

doi:10.1039/d0ta01680b

	Activation strategies of water-splitting electrocatalysts
	Liu, Peng Fei 2; Yin, Huajie 1; Fu, Huai Qin 1,2; Zu, Meng Yang 2; Yang, Hua Gui 2; Zhao, Huijun 1,3
刊名	JOURNAL OF MATERIALS CHEMISTRY A
	2020-05-28
卷号	8
ISSN号	2050-7488
DOI	10.1039/d0ta01680b
通讯作者	Yang, Hua Gui(hgyang@ecust.edu.cn) ; Zhao, Huijun(h.zhao@griffith.edu.au)
英文摘要	Electrocatalysts featuring high activity, selectivity and stability are urgently needed in solar-electricity powered energy-conversion technologies. In the past decade, various electrocatalysts have been demonstrated to be electrocatalytically active toward the hydrogen evolution reaction (HER) and oxygen evolution reaction (OER). Despite the significant progress, catalyst discovery is still dominated by "trial-and-error" practice due to the lack of understanding of the origin of electrocatalytic activity, active site structures and key factors determining the operando electrocatalytic performance. Therefore, this critical review focuses on summarizing effective catalyst activation strategies to enable efficient catalyst discovery, on the basis of understanding real active sites for the HER and OER. Meanwhile, theory prediction and operando characterization techniques have also been introduced to identify the origin of electrocatalytic activity and active site structures. Moreover, catalyst atomic structure reconstruction/rearrangement under working conditions and the accompanying catalyst activation strategies have been discussed to address the negative impacts of reaction media. Finally, a brief perspective on the challenges and future directions for predicting, characterizing and understanding operando active sites to discover efficient activation strategies will also be presented.
资助项目	Australian Research Council (ARC) Discovery Project[DP170104834] ; National Natural Science Funds for Distinguished Young Scholar[51725201] ; International (Regional) Cooperation and Exchange Projects of the National Natural Science Foundation of China[51920105003] ; Innovation Program of Shanghai Municipal Education Commission[E00014] ; National Natural Science Foundation of China[21573068] ; National Natural Science Foundation of China[51902105] ; Shanghai Engineering Research Center of Hierarchical Nanomaterials[18DZ2252400] ; Shanghai Sailing Program[19YF1411600] ; China Postdoctoral Science Foundation[2018M641938] ; Griffith University Postdoctoral Fellowship
WOS关键词	HYDROGEN EVOLUTION REACTION ; LAYERED DOUBLE HYDROXIDE ; HIGHLY-ACTIVE ELECTROCATALYST ; AMORPHOUS MOLYBDENUM SULFIDE ; RAY-ABSORPTION SPECTROSCOPY ; ENHANCED CATALYTIC-ACTIVITY ; OXYGEN EVOLUTION ; SINGLE-ATOM ; PEROVSKITE ELECTROCATALYST ; EFFICIENT ELECTROCATALYSTS
WOS研究方向	Chemistry ; Energy & Fuels ; Materials Science
语种	英语
出版者	ROYAL SOC CHEMISTRY
WOS记录号	WOS:000539350100003
资助机构	Australian Research Council (ARC) Discovery Project ; National Natural Science Funds for Distinguished Young Scholar ; International (Regional) Cooperation and Exchange Projects of the National Natural Science Foundation of China ; Innovation Program of Shanghai Municipal Education Commission ; National Natural Science Foundation of China ; Shanghai Engineering Research Center of Hierarchical Nanomaterials ; Shanghai Sailing Program ; China Postdoctoral Science Foundation ; Griffith University Postdoctoral Fellowship
内容类型	期刊论文
源URL	[http://ir.hfcas.ac.cn:8080/handle/334002/102983]
专题	中国科学院合肥物质科学研究院
通讯作者	Yang, Hua Gui; Zhao, Huijun
作者单位	1.Griffith Univ, Ctr Clean Environm & Energy, Gold Coast Campus, Gold Coast, Qld 4222, Australia 2.East China Univ Sci & Technol, Shanghai Engn Res Ctr Hierarch Nanomat, Sch Mat Sci & Engn, Key Lab Ultrafine Mat,Minist Educ, Shanghai 200237, Peoples R China 3.Chinese Acad Sci, Inst Solid State Phys, CAS Ctr Excellence Nanosci, Ctr Environm & Energy Nanomat, Hefei 230031, Peoples R China
推荐引用方式 GB/T 7714	Liu, Peng Fei,Yin, Huajie,Fu, Huai Qin,et al. Activation strategies of water-splitting electrocatalysts[J]. JOURNAL OF MATERIALS CHEMISTRY A,2020,8.
APA	Liu, Peng Fei,Yin, Huajie,Fu, Huai Qin,Zu, Meng Yang,Yang, Hua Gui,&Zhao, Huijun.(2020).Activation strategies of water-splitting electrocatalysts.JOURNAL OF MATERIALS CHEMISTRY A,8.
MLA	Liu, Peng Fei,et al."Activation strategies of water-splitting electrocatalysts".JOURNAL OF MATERIALS CHEMISTRY A 8(2020).