Effect of the interaction strength and anisotropy on the diffusio-phoresis of spherical colloids | |
Wei JC(韦佳辰)3,4; Ramirez-Hinestrosa S3; Dobnikar J1,2,3; Frenkel D3 | |
刊名 | SOFT MATTER |
2020-04-21 | |
卷号 | 16期号:15页码:3621-3627 |
ISSN号 | 1744-683X |
DOI | 10.1039/c9sm02053e |
通讯作者 | Dobnikar, Jure(jd489@cam.ac.uk) ; Frenkel, Daan(df246@cam.ac.uk) |
英文摘要 | Gradients in temperature, concentration or electrostatic potential cannot exert forces on a bulk fluid; they can, however, exert forces on a fluid in a microscopic boundary layer surrounding a (nano)colloidal solute, resulting in so-called phoretic flow. Here we present a simulation study of phoretic flow around a spherical colloid held fixed in a concentration gradient. We show that the resulting flow velocity depends non-monotonically on the strength of the colloid-fluid interaction. The reason for this non-monotonic dependence is that solute particles are effectively trapped in a shell around the colloid and cannot contribute to diffusio-phoresis. We also observe that the flow depends sensitively on the anisotropy of solute-colloid interaction. |
分类号 | 二类/Q1 |
资助项目 | National Key Research and Development Program of China[2016YFA0501601] ; EU[766972-FET-OPEN-NANOPHLOW] ; K. C. Wong Educational Foundation ; National Natural Science Foundations of China[11602279] ; National Natural Science Foundations of China[11874398] |
WOS关键词 | PARTICLES ; GRADIENTS ; THERMOPHORESIS ; MIGRATION ; SALT |
WOS研究方向 | Chemistry ; Materials Science ; Physics ; Polymer Science |
语种 | 英语 |
WOS记录号 | WOS:000527020700020 |
资助机构 | National Key Research and Development Program of China ; EU ; K. C. Wong Educational Foundation ; National Natural Science Foundations of China |
其他责任者 | Dobnikar, Jure ; Frenkel, Daan |
内容类型 | 期刊论文 |
源URL | [http://dspace.imech.ac.cn/handle/311007/81879] |
专题 | 力学研究所_非线性力学国家重点实验室 |
作者单位 | 1.Songshan Lake Mat Lab, Dongguan 523808, Peoples R China 2.Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China; 3.Univ Cambridge, Dept Chem, Cambridge CB2 1EW, England; 4.Chinese Acad Sci, Inst Mech, Beijing 100190, Peoples R China; |
推荐引用方式 GB/T 7714 | Wei JC,Ramirez-Hinestrosa S,Dobnikar J,et al. Effect of the interaction strength and anisotropy on the diffusio-phoresis of spherical colloids[J]. SOFT MATTER,2020,16(15):3621-3627. |
APA | 韦佳辰,Ramirez-Hinestrosa S,Dobnikar J,&Frenkel D.(2020).Effect of the interaction strength and anisotropy on the diffusio-phoresis of spherical colloids.SOFT MATTER,16(15),3621-3627. |
MLA | 韦佳辰,et al."Effect of the interaction strength and anisotropy on the diffusio-phoresis of spherical colloids".SOFT MATTER 16.15(2020):3621-3627. |
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