Effect of dissolved organic matters on adsorption and desorption behavior of heavy metals in a water-level-fluctuation zone of the Three Gorges Reservoir, China | |
Huang, Yang3,4; Fu, Chuan2; Li, Zhe1; Fang, Fang3; Ouyang, Wenjuan1; Guo, Jinsong3 | |
刊名 | ECOTOXICOLOGY AND ENVIRONMENTAL SAFETY |
2019-12-15 | |
卷号 | 185页码:7 |
关键词 | Water-level-fluctuating zone Dissolved organic matter Cd adsorption-desorption Cr adsorption-desorption Cu adsorption-desorption |
ISSN号 | 0147-6513 |
DOI | 10.1016/j.ecoenv.2019.109695 |
通讯作者 | Guo, Jinsong(guo0768@cqu.edu.cn) |
英文摘要 | Operation of recession and inundation in Three Gorges Reservoir (TGR) revealed a potential contribution to the migration of heavy metals in soil and fluvial systems, thus led to negative ecological impacts. The work herein investigated the concentration and speciation of three typical heavy metals (Cd, Cr and Cu) in a water-level-fluctuation zone of TGR, as well as simulated the adsorption and desorption behavior of heavy metals on soils, which aimed at elucidating the fate of heavy metals in this special area. Field investigation revealed that water level fluctuation greatly enabled the migration of heavy metals to inner or upper soil layers. Laboratory experiments showed that adsorption of Cd(II) was a chemical process and dissolved organic matters (DOM) in soils strengthened the combination of Cd(II) to soil surface which inhibited the desorption process. Cr(VI) was physically adsorbed and readily to be desorbed. DOM enabled deposition of Cr(VI) in soils. Cation exchange was dominate mechanism in Cu(II) adsorption process, whereas DOM presented positive effects on desorption of Cu (II). The results presented in this study would provide basic theory for scientific research in TGR. |
资助项目 | National Natural Science Foundation of China[41771520] ; National Natural Science Foundation of China[41430750] ; National Natural Science Foundation of China[51708050] ; Chengdu University of Information Technology[KYTZ201739] ; Chengdu University of Information Technology[CRF201707] |
WOS研究方向 | Environmental Sciences & Ecology ; Toxicology |
语种 | 英语 |
出版者 | ACADEMIC PRESS INC ELSEVIER SCIENCE |
WOS记录号 | WOS:000491218500045 |
内容类型 | 期刊论文 |
源URL | [http://119.78.100.138/handle/2HOD01W0/9665] |
专题 | 中国科学院重庆绿色智能技术研究院 |
通讯作者 | Guo, Jinsong |
作者单位 | 1.Chinese Acad Sci, Chongqing Inst Green & Intelligent Technol, Key Lab Reservoir Environm, Chongqing 400714, Peoples R China 2.Chongqing Three Gorges Univ, Coll Chem & Environm Engn, Chongqing 404000, Peoples R China 3.Chongqing Univ, MOE, Key Lab Three Gorges Reservoir Reg Ecoenvironm, Chongqing 400045, Peoples R China 4.Chengdu Univ Informat Technol, Coll Resources & Environm, Chengdu 610225, Sichuan, Peoples R China |
推荐引用方式 GB/T 7714 | Huang, Yang,Fu, Chuan,Li, Zhe,et al. Effect of dissolved organic matters on adsorption and desorption behavior of heavy metals in a water-level-fluctuation zone of the Three Gorges Reservoir, China[J]. ECOTOXICOLOGY AND ENVIRONMENTAL SAFETY,2019,185:7. |
APA | Huang, Yang,Fu, Chuan,Li, Zhe,Fang, Fang,Ouyang, Wenjuan,&Guo, Jinsong.(2019).Effect of dissolved organic matters on adsorption and desorption behavior of heavy metals in a water-level-fluctuation zone of the Three Gorges Reservoir, China.ECOTOXICOLOGY AND ENVIRONMENTAL SAFETY,185,7. |
MLA | Huang, Yang,et al."Effect of dissolved organic matters on adsorption and desorption behavior of heavy metals in a water-level-fluctuation zone of the Three Gorges Reservoir, China".ECOTOXICOLOGY AND ENVIRONMENTAL SAFETY 185(2019):7. |
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