Thickness-driven first-order phase transitions in manganite ultrathin films | |
Chen, HY; Yu, Y; Wang, Z; Bai, Y; Lin, HX; Li, XL; Liu, H; Miao, T; Kou, YF; Zhang, YS | |
刊名 | PHYSICAL REVIEW B |
2019 | |
卷号 | 99期号:21页码:— |
关键词 | TOTAL-ENERGY CALCULATIONS GIANT MAGNETORESISTANCE |
ISSN号 | 2469-9950 |
DOI | 10.1103/PhysRevB.99.214419 |
文献子类 | 期刊论文 |
英文摘要 | We report thickness dependent inhomogeneous antiferromagnetic (AFM) to ferromagnetic (FM) phase transitions in ultrathin La0.7Sr0.3MnO3 (LSMO) films grown on the SrTiO3 substrate. When the films are 4-7 unit cells (UCs) thick, FM domains appear as isolated nanodisks in the AFM matrix that together floats on top of the three AFM base UCs, leading a superparamagnetic blocking behavior. Our first principles calculations unravel the rather counterintuitive physical origin of this mixed phase state; the formation of FM/AFM domain boundaries is energetically favorable. At 8 UCs, an abrupt shear strain relief occurs in the LSMO thin film and twinning patterns with two unit cell periodicity form along the [010] and [100] directions. Our studies reveal the complexity of the magnetic phase transition at the nanometer scale and open a door for the development of quantum devices and statistical theories. |
语种 | 英语 |
内容类型 | 期刊论文 |
源URL | [http://ir.sinap.ac.cn/handle/331007/31876] |
专题 | 上海应用物理研究所_中科院上海应用物理研究所2011-2017年 |
作者单位 | 1.Fudan Univ, State Key Lab Surface Phys, Shanghai 200433, Peoples R China; 2.Fudan Univ, Dept Phys, Shanghai 200433, Peoples R China; 3.Fudan Univ, Inst Nanoelect Devices & Quantum Comp, Shanghai 200433, Peoples R China; 4.Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China; 5.Nanjing Univ, Collaborat Innovat Ctr Adv Microstruct, Nanjing 210093, Jiangsu, Peoples R China; 6.Tsinghua Univ, Natl Ctr Electron Microscopy Beijing, Sch Mat Sci & Engn, Key Lab Adv Mat MOE,State Key Lab New Ceram & Fin, Beijing 100084, Peoples R China; 7.Chinese Acad Sci, Shanghai Inst Appl Phys, Shanghai 201204, Peoples R China |
推荐引用方式 GB/T 7714 | Chen, HY,Yu, Y,Wang, Z,et al. Thickness-driven first-order phase transitions in manganite ultrathin films[J]. PHYSICAL REVIEW B,2019,99(21):—. |
APA | Chen, HY.,Yu, Y.,Wang, Z.,Bai, Y.,Lin, HX.,...&Shen, J.(2019).Thickness-driven first-order phase transitions in manganite ultrathin films.PHYSICAL REVIEW B,99(21),—. |
MLA | Chen, HY,et al."Thickness-driven first-order phase transitions in manganite ultrathin films".PHYSICAL REVIEW B 99.21(2019):—. |
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