A perspective on two-dimensional materials for planar micro-supercapacitors

doi:10.1063/1.5113940

	A perspective on two-dimensional materials for planar micro-supercapacitors
	Qin, Jieqiong 1,2; Das, Pratteek 1,2; Zheng, Shuanghao 1,2,3; Wu, Zhong-Shuai 2
刊名	APL MATERIALS
	2019-09-01
卷号	7 期号:9 页码:17
ISSN号	2166-532X
DOI	10.1063/1.5113940
通讯作者	Wu, Zhong-Shuai(wuzs@dicp.ac.cn)
英文摘要	The increasing demand for portable, wearable, and miniaturized electronics has substantially promoted the immense development of planar microsupercapacitors (MSCs) built on a single substrate. Atomically thin two-dimensional (2D) nanosheets, by virtue of their intrinsically unique structure and fascinating electrochemical properties, provide a new material platform for the creation of high performance planar MSCs in which the electrolyte ions can completely utilize flat architecture and ultrathin thickness of 2D nanosheets, parallel to the direction of ionic diffusion along the plane of 2D nanosheets. Herein, we present an overview and perspective on diverse 2D materials for planar MSCs. First, an introduction is presented to highlight the advances of MSCs, the uniqueness of 2D materials in the assembly of planar MSCs with three different configurations, i.e., stacked, interdigital, and 3D planar geometries, and the progress of microfabrication techniques for microelectrodes of MSCs. Second, the state-of-the-art 2D materials to manufacture planar MSCs, including graphene, transition metal oxides/hydroxides, transition metal dichalcogenides, metal carbides, metal nitrides, phosphorene, boron nitride, metal-organic frameworks, and covalent-organic frameworks, are systemically discussed in detail. Special emphasis is given to the multiple roles of 2D materials for functional components as active materials, current collectors, additives/binders, and separators for planar MSCs. Finally, the existing challenges and prospective solutions of 2D materials for planar MSCs with high performance and various innovative form factors are proposed.
资助项目	National Natural Science Foundation of China[51702078] ; National Natural Science Foundation of China[51572259] ; National Natural Science Foundation of China[51872283] ; National Key R&D Program of China[2016YFB0100100] ; National Key R&D Program of China[2016YFA0200200] ; Natural Science Foundation of Liaoning Province[20180510038] ; LiaoNing Revitalization Talents Program[XLYC1807153] ; DICP[DICP ZZBS201708] ; DICP[DICP ZZBS201802] ; DICPQIBEBT[DICPQIBEBT UN201702] ; Dalian National Laboratory for Clean Energy (DNL), CAS ; DNL Cooperation Fund, CAS[DNL180310] ; DNL Cooperation Fund, CAS[DNL180308]
WOS关键词	ALL-SOLID-STATE ; ULTRAHIGH VOLUMETRIC CAPACITANCE ; COVALENT ORGANIC FRAMEWORK ; GRAPHENE-BASED MATERIALS ; METAL-OXIDE NANOSHEETS ; HIGH-PERFORMANCE ; ENERGY-STORAGE ; RECENT PROGRESS ; HIGH-VOLTAGE ; HIGH AREAL
WOS研究方向	Science & Technology - Other Topics ; Materials Science ; Physics
语种	英语
出版者	AMER INST PHYSICS
WOS记录号	WOS:000489245900017
资助机构	National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Key R&D Program of China ; National Key R&D Program of China ; Natural Science Foundation of Liaoning Province ; Natural Science Foundation of Liaoning Province ; LiaoNing Revitalization Talents Program ; LiaoNing Revitalization Talents Program ; DICP ; DICP ; DICPQIBEBT ; DICPQIBEBT ; Dalian National Laboratory for Clean Energy (DNL), CAS ; Dalian National Laboratory for Clean Energy (DNL), CAS ; DNL Cooperation Fund, CAS ; DNL Cooperation Fund, CAS ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Key R&D Program of China ; National Key R&D Program of China ; Natural Science Foundation of Liaoning Province ; Natural Science Foundation of Liaoning Province ; LiaoNing Revitalization Talents Program ; LiaoNing Revitalization Talents Program ; DICP ; DICP ; DICPQIBEBT ; DICPQIBEBT ; Dalian National Laboratory for Clean Energy (DNL), CAS ; Dalian National Laboratory for Clean Energy (DNL), CAS ; DNL Cooperation Fund, CAS ; DNL Cooperation Fund, CAS ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Key R&D Program of China ; National Key R&D Program of China ; Natural Science Foundation of Liaoning Province ; Natural Science Foundation of Liaoning Province ; LiaoNing Revitalization Talents Program ; LiaoNing Revitalization Talents Program ; DICP ; DICP ; DICPQIBEBT ; DICPQIBEBT ; Dalian National Laboratory for Clean Energy (DNL), CAS ; Dalian National Laboratory for Clean Energy (DNL), CAS ; DNL Cooperation Fund, CAS ; DNL Cooperation Fund, CAS ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Key R&D Program of China ; National Key R&D Program of China ; Natural Science Foundation of Liaoning Province ; Natural Science Foundation of Liaoning Province ; LiaoNing Revitalization Talents Program ; LiaoNing Revitalization Talents Program ; DICP ; DICP ; DICPQIBEBT ; DICPQIBEBT ; Dalian National Laboratory for Clean Energy (DNL), CAS ; Dalian National Laboratory for Clean Energy (DNL), CAS ; DNL Cooperation Fund, CAS ; DNL Cooperation Fund, CAS
内容类型	期刊论文
源URL	[http://cas-ir.dicp.ac.cn/handle/321008/172510]
专题	大连化学物理研究所_中国科学院大连化学物理研究所
通讯作者	Wu, Zhong-Shuai
作者单位	1.Univ Chinese Acad Sci, 19 A Yuquan Rd, Beijing 100049, Peoples R China 2.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, 457 Zhongshan Rd, Dalian 116023, Peoples R China 3.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, 457 Zhongshan Rd, Dalian 116023, Peoples R China
推荐引用方式 GB/T 7714	Qin, Jieqiong,Das, Pratteek,Zheng, Shuanghao,et al. A perspective on two-dimensional materials for planar micro-supercapacitors[J]. APL MATERIALS,2019,7(9):17.
APA	Qin, Jieqiong,Das, Pratteek,Zheng, Shuanghao,&Wu, Zhong-Shuai.(2019).A perspective on two-dimensional materials for planar micro-supercapacitors.APL MATERIALS,7(9),17.
MLA	Qin, Jieqiong,et al."A perspective on two-dimensional materials for planar micro-supercapacitors".APL MATERIALS 7.9(2019):17.