Effective TiO2 hybrid heterostructure fabricated on nano mesoporous phenolic resol for visible-light photocatalysis
Jiang, Yijun; Meng, Lingqian; Mu, Xindong; Li, Xiutao; Wang, Haisong; Chen, Xiufang; Wang, Xicheng; Wang, Wei; Wu, Feng; Wang, Xiaoyan
刊名JOURNAL OF MATERIALS CHEMISTRY
2012-11-28
卷号22期号:44页码:23642-23649
中文摘要 Highly homogeneous TiO2@phenolic resol hybrid nanocomposites are fabricated by a solvothermal method. In such nanostructures, the TiO2 particles are tightly grafted on the surface of nano mesoporous phenolic resols to form uniform heterostructures. Significantly, a charge transfer complex was formed at the interface of the TiO2 and the nano mesoporous phenolic resols, which led to visiblelight absorption over the full range. The nano hybrid material exhibited excellent performance for the photocatalytic degradation of dyes and produced photocurrent signals under visible-light. The investigation of the mechanism indicated that the O2_ was the main active species during the photochemical process. The hybrid nanocomposites also showed considerably high stability in the photocatalysis. It is expected that this approach can provide a new strategy for the design of some bio-inspired catalysts for sustainable technology.
英文摘要Highly homogeneous TiO2@phenolic resol hybrid nanocomposites are fabricated by a solvothermal method. In such nanostructures, the TiO2 particles are tightly grafted on the surface of nano mesoporous phenolic resols to form uniform heterostructures. Significantly, a charge transfer complex was formed at the interface of the TiO2 and the nano mesoporous phenolic resols, which led to visible-light absorption over the full range. The nano hybrid material exhibited excellent performance for the photocatalytic degradation of dyes and produced photocurrent signals under visible-light. The investigation of the mechanism indicated that the O-2(-) was the main active species during the photochemical process. The hybrid nanocomposites also showed considerably high stability in the photocatalysis. It is expected that this approach can provide a new strategy for the design of some bio-inspired catalysts for sustainable technology.
学科主题绿色化学催化
WOS标题词Science & Technology ; Physical Sciences ; Technology
类目[WOS]Chemistry, Physical ; Materials Science, Multidisciplinary
研究领域[WOS]Chemistry ; Materials Science
关键词[WOS]TITANIUM-DIOXIDE ; CHARGE-TRANSFER ; FUEL-CELL ; NANOPARTICLES ; GENERATION ; COMPLEX ; RESIN ; MECHANISMS ; DYNAMICS ; POWDERS
收录类别SCI
语种英语
WOS记录号WOS:000310934400045
公开日期2012-11-16
内容类型期刊论文
源URL[http://ir.qibebt.ac.cn:8080/handle/337004/1402]  
专题青岛生物能源与过程研究所_绿色化学催化团队
作者单位Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Key Lab Biofuels, Qingdao 266101, Peoples R China
推荐引用方式
GB/T 7714
Jiang, Yijun,Meng, Lingqian,Mu, Xindong,et al. Effective TiO2 hybrid heterostructure fabricated on nano mesoporous phenolic resol for visible-light photocatalysis[J]. JOURNAL OF MATERIALS CHEMISTRY,2012,22(44):23642-23649.
APA Jiang, Yijun.,Meng, Lingqian.,Mu, Xindong.,Li, Xiutao.,Wang, Haisong.,...&Wang, Xiaoyan.(2012).Effective TiO2 hybrid heterostructure fabricated on nano mesoporous phenolic resol for visible-light photocatalysis.JOURNAL OF MATERIALS CHEMISTRY,22(44),23642-23649.
MLA Jiang, Yijun,et al."Effective TiO2 hybrid heterostructure fabricated on nano mesoporous phenolic resol for visible-light photocatalysis".JOURNAL OF MATERIALS CHEMISTRY 22.44(2012):23642-23649.
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