Assessing and Forecasting Atmospheric Outflow of alpha-HCH from China on Intra-, Inter-, and Decadal Time Scales

CORC > 烟台海岸带研究所 > 中国科学院烟台海岸带研究所 > 中科院海岸带环境过程与生态修复重点实验室 > 污染过程与控制实验室

	Assessing and Forecasting Atmospheric Outflow of alpha-HCH from China on Intra-, Inter-, and Decadal Time Scales
	Tian, Chongguo1,2,3 ; Ma, Jianmin 4; Chen, Yingjun 1,2; Liu, Liyan 3; Ma, Wanli 3; Li, Yi-Fan 3,4
刊名	ENVIRONMENTAL SCIENCE & TECHNOLOGY
	2012-02-21
卷号	46 期号:4 页码:2220-2227
关键词	POLYCYCLIC AROMATIC-HYDROCARBONS CLIMATE-CHANGE TECHNICAL HEXACHLOROCYCLOHEXANE ORGANOCHLORINE PESTICIDES TRANSPACIFIC TRANSPORT SEASONAL-VARIATIONS ASIAN POLLUTION AIR-POLLUTION PACIFIC PATHWAYS
ISSN号	0013-936X
通讯作者	Tian, CG (reprint author), Chinese Acad Sci, Key Lab Coastal Zone Environm Proc, Yantai Inst Coastal Zone Res, Yantai 264003, Shandong, Peoples R China. cgtian@yic.ac.cn
产权排序	[Tian, Chongguo; Chen, Yingjun] Chinese Acad Sci, Key Lab Coastal Zone Environm Proc, Yantai Inst Coastal Zone Res, Yantai 264003, Shandong, Peoples R China; [Tian, Chongguo; Chen, Yingjun] YICCAS, Shandong Prov Key Lab Coastal Zone Environm Proc, Yantai 264003, Shandong, Peoples R China; [Tian, Chongguo; Liu, Liyan; Ma, Wanli; Li, Yi-Fan] Harbin Inst Technol, Int Joint Res Ctr Persistent Tox Subst, State Key Lab Urban Water Resource & Environm, Harbin 150090, Peoples R China; [Ma, Jianmin; Li, Yi-Fan] Environm Canada, Air Qual Res Div, Sci & Technol Branch, Toronto, ON M3H 5T4, Canada
中文摘要	Atmospheric outflow of alpha-HCH-HCH from China from 1952 to 2009 was investigated using Chinese Gridded Pesticide Emission and Residue Model (ChnGPERM). The model results show that the outflows via the northeast boundary (NEB, longitude 115-135 degrees E along 55 degrees N and latitude 37-55 degrees N along 135 degrees E) and the mid-south boundary (MSB, longitude 100-120 degrees E along 17 degrees N) of China account for 47% and 35% of the total outflow, respectively. Two climate indices based on the statistical association between the time series of modeled alpha-HCH outflow and atmospheric sea-level pressure were developed to predict the outflow on different time scales. The first index explains 70/83% and 10/46% of the intra-annual variability of the outflow via the NEB and MSB during the periods of 1952-1984 and 1985-2009, respectively. The second index explains 16% and 19% of the interannual and longer time scale variability in the outflow through the NEB during June-August and via the MSB during October December for 1991-2009, respectively. Results also revealed that climate warming may potentially result in stronger outflow via the NEB than the MSB. The linkage between the outflow with large scale atmospheric circulation patterns and climate warming trend over China was also discussed.
英文摘要	Atmospheric outflow of alpha-HCH-HCH from China from 1952 to 2009 was investigated using Chinese Gridded Pesticide Emission and Residue Model (ChnGPERM). The model results show that the outflows via the northeast boundary (NEB, longitude 115-135 degrees E along 55 degrees N and latitude 37-55 degrees N along 135 degrees E) and the mid-south boundary (MSB, longitude 100-120 degrees E along 17 degrees N) of China account for 47% and 35% of the total outflow, respectively. Two climate indices based on the statistical association between the time series of modeled alpha-HCH outflow and atmospheric sea-level pressure were developed to predict the outflow on different time scales. The first index explains 70/83% and 10/46% of the intra-annual variability of the outflow via the NEB and MSB during the periods of 1952-1984 and 1985-2009, respectively. The second index explains 16% and 19% of the interannual and longer time scale variability in the outflow through the NEB during June-August and via the MSB during October December for 1991-2009, respectively. Results also revealed that climate warming may potentially result in stronger outflow via the NEB than the MSB. The linkage between the outflow with large scale atmospheric circulation patterns and climate warming trend over China was also discussed.
学科主题	Engineering; Environmental Sciences & Ecology
研究领域[WOS]	Engineering ; Environmental Sciences & Ecology
关键词[WOS]	POLYCYCLIC AROMATIC-HYDROCARBONS ; CLIMATE-CHANGE ; TECHNICAL HEXACHLOROCYCLOHEXANE ; ORGANOCHLORINE PESTICIDES ; TRANSPACIFIC TRANSPORT ; SEASONAL-VARIATIONS ; ASIAN POLLUTION ; AIR-POLLUTION ; PACIFIC ; PATHWAYS
收录类别	SCI
资助信息	Chinese Academy of Sciences[KZCX2-YW-GJ02]; State Key Laboratory of Urban Water Resource and Environment, Harbin Institute of Technology[HC201019]; Natural Scientific Foundation of China[41101495, 40806048]
原文出处	http://pubs.acs.org/doi/pdfplus/10.1021/es202851n
语种	英语
WOS记录号	WOS:000300465900034
公开日期	2012-06-13
内容类型	期刊论文
源URL	[http://ir.yic.ac.cn/handle/133337/5600]
专题	烟台海岸带研究所_污染过程与控制实验室
作者单位	1.Chinese Acad Sci, Key Lab Coastal Zone Environm Proc, Yantai Inst Coastal Zone Res, Yantai 264003, Shandong, Peoples R China 2.YICCAS, Shandong Prov Key Lab Coastal Zone Environm Proc, Yantai 264003, Shandong, Peoples R China 3.Harbin Inst Technol, Int Joint Res Ctr Persistent Tox Subst, State Key Lab Urban Water Resource & Environm, Harbin 150090, Peoples R China 4.Environm Canada, Air Qual Res Div, Sci & Technol Branch, Toronto, ON M3H 5T4, Canada
推荐引用方式 GB/T 7714	Tian, Chongguo,Ma, Jianmin,Chen, Yingjun,et al. Assessing and Forecasting Atmospheric Outflow of alpha-HCH from China on Intra-, Inter-, and Decadal Time Scales[J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY,2012,46(4):2220-2227.
APA	Tian, Chongguo,Ma, Jianmin,Chen, Yingjun,Liu, Liyan,Ma, Wanli,&Li, Yi-Fan.(2012).Assessing and Forecasting Atmospheric Outflow of alpha-HCH from China on Intra-, Inter-, and Decadal Time Scales.ENVIRONMENTAL SCIENCE & TECHNOLOGY,46(4),2220-2227.
MLA	Tian, Chongguo,et al."Assessing and Forecasting Atmospheric Outflow of alpha-HCH from China on Intra-, Inter-, and Decadal Time Scales".ENVIRONMENTAL SCIENCE & TECHNOLOGY 46.4(2012):2220-2227.