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Characterization of HCHs and DDTs in urban dustfall and prediction of soil burden in a metropolis-Beijing, China
Cheng, HX (Cheng, Hangxin); Ma, LL (Ma, Lingling); Zhao, CD (Zhao, Chuandong); Li, XH (Li, Xinghong); Wang, XF (Wang, Xiaofei); Liu, YH (Liu, Yinghan); Yang, K (Yang, Ke)
刊名CHEMOSPHERE
2011
卷号85期号:3页码:406-411
关键词HCHs DDTs Dustfall Flux Fugacity
ISSN号0045-6535
英文摘要The concentrations, spatial distribution and compositional patterns of extensively used hexachlorocyclohexanes (HCHs) and dichlorodiphenyltrichloroethanes (DDTs) in urban dustfall in a metropolis-Beijing are presented in this paper. The potential sources are discussed and soil burdens are predicted based on the fluxes. The hotspots in commercial areas are identified by spatial distribution maps and the fractional value isomers indicates that dustfall in urban Beijing are affected by both current and historical usage of DDTs. It is worth noticing that there is possible application "dicofol-type of DDTs" in Beijing. The measured atmospheric deposition flux is 1.14 x 10(5) ng h(-1) m(-2) for HCHs and 1.47 x 10(5) ng h(-1) m(-2) for DDTs, respectively. However, when compared with atmospheric deposition flux, the volatilization flux estimated from concentrations in soils by fugacity model is significantly lower for HCHs (2.41 ng h(-1) m(-2)) and DDTs (0.07 ng h(-1) m(-2)). The net atmospheric flux to the soil suggests that the levels of HCHs and DDTs in soil are dominated by atmospheric deposition and the urban soil in Beijing would be a sink for HCHs and DDTs in the long term. Crown Copyright (C) 2011 Published by Elsevier Ltd. All rights reserved.
学科主题环境地质学
WOS关键词PERSISTENT ORGANIC POLLUTANTS ; ORGANOCHLORINE PESTICIDES ; TECHNICAL HEXACHLOROCYCLOHEXANE ; POLYCHLORINATED-BIPHENYLS ; AIR ; CANADA ; FATE ; OUTSKIRTS ; RESIDUES ; TRENDS
WOS研究方向Environmental Sciences & Ecology
语种英语
出版者PERGAMON-ELSEVIER SCIENCE LTD
WOS记录号WOS:000297661900017
内容类型期刊论文
源URL[http://119.78.100.197/handle/2HKVOGP0/39457]  
专题中国地质调查局
作者单位Chinese Acad Sci, Res Ctr Ecoenvironm Sci, State Key Lab Environm Chem & Ecotoxicol, Beijing 100085, Peoples R China
推荐引用方式
GB/T 7714
Cheng, HX ,Ma, LL ,Zhao, CD ,et al. Characterization of HCHs and DDTs in urban dustfall and prediction of soil burden in a metropolis-Beijing, China[J]. CHEMOSPHERE,2011,85(3):406-411.
APA Cheng, HX .,Ma, LL .,Zhao, CD .,Li, XH .,Wang, XF .,...&Yang, K .(2011).Characterization of HCHs and DDTs in urban dustfall and prediction of soil burden in a metropolis-Beijing, China.CHEMOSPHERE,85(3),406-411.
MLA Cheng, HX ,et al."Characterization of HCHs and DDTs in urban dustfall and prediction of soil burden in a metropolis-Beijing, China".CHEMOSPHERE 85.3(2011):406-411.
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