High-Mobility p-Type Organic Semiconducting Interlayer Enhancing Efficiency and Stability of Perovskite Solar Cells | |
Zhang, Mingyu ; Wang, Jiayu ; Li, Liang ; Zheng, Guanhaojie ; Liu, Kuan ; Qin, Meng ; Zhou, Huanping ; Zhan, Xiaowei | |
刊名 | ADVANCED SCIENCE |
2017 | |
关键词 | high mobility interlayers organic semiconductors perovskite solar cells p-type ORGANOMETAL HALIDE PEROVSKITES HOLE-TRANSPORTING MATERIAL PERFORMANCE LENGTHS CH3NH3PBI3 DEPOSITION LAYERS |
DOI | 10.1002/advs.201700025 |
英文摘要 | A high-mobility p-type organic semiconductor based on benzodithiophene and diketopyrrolopyrrole with linear alkylthio substituents (BDTS-2DPP) is used as a dual function interfacial layer to modify the interface of perovskite/2,2',7,7'-tetrakis(N,N'-di-p-methoxyphenylamine)-9,9'-spirobifluorene in planar perovskite solar cells. The BDTS-2DPP layer can remarkably passivate the surface defects of perovskite through the formation of Lewis adduct between the under-coordinated Pb atoms in perovskite and S atoms in BDTS-2DPP, and also shows efficient hole extraction and transfer properties. The devices with BDTS-2DPP interlayer show a peak power conversion efficiency of 18.2%, which is higher than that of reference devices without the BDTS-2DPP interlayer (16.9%). Moreover, the hydrophobic BDTS-2DPP interlayer effectively protects the perovskite against moisture, leading to enhanced device stability.; NSFC [21673011]; SCI(E); ARTICLE; 9; 4 |
语种 | 英语 |
内容类型 | 期刊论文 |
源URL | [http://ir.pku.edu.cn/handle/20.500.11897/471051] |
专题 | 工学院 |
推荐引用方式 GB/T 7714 | Zhang, Mingyu,Wang, Jiayu,Li, Liang,et al. High-Mobility p-Type Organic Semiconducting Interlayer Enhancing Efficiency and Stability of Perovskite Solar Cells[J]. ADVANCED SCIENCE,2017. |
APA | Zhang, Mingyu.,Wang, Jiayu.,Li, Liang.,Zheng, Guanhaojie.,Liu, Kuan.,...&Zhan, Xiaowei.(2017).High-Mobility p-Type Organic Semiconducting Interlayer Enhancing Efficiency and Stability of Perovskite Solar Cells.ADVANCED SCIENCE. |
MLA | Zhang, Mingyu,et al."High-Mobility p-Type Organic Semiconducting Interlayer Enhancing Efficiency and Stability of Perovskite Solar Cells".ADVANCED SCIENCE (2017). |
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