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Alignment-Dependent Fluorescence Emission Induced by Tunnel Ionization of Carbon Dioxide from Lower-Lying Orbitals
Yao, Jinping ; Li, Guihua ; Jia, Xinyan ; Hao, Xiaolei ; Zeng, Bin ; Jing, Chenrui ; Chu, Wei ; Ni, Jielei ; Zhang, Haisu ; Xie, Hongqiang ; Zhang, Chaojin ; Zhao, Zengxiu ; Chen, Jing ; Liu, Xiaojun ; Cheng, Ya ; Xu, Zhizhan
刊名物理评论快报
2013
关键词HARMONIC-GENERATION MULTIPLE ORBITALS LASER FIELDS MOLECULES DYNAMICS
DOI10.1103/PhysRevLett.111.133001
英文摘要The study of the ionization process of molecules in an intense infrared laser field is of paramount interest in strong-field physics and constitutes the foundation of imaging of molecular valence orbitals and attosecond science. We show measurement of alignment-dependent ionization probabilities of the lower-lying orbitals of the molecules by experimentally detecting the alignment dependence of fluorescence emission from tunnel ionized carbon dioxide molecules. The experimental measurements are compared with the theoretical calculations of the strong field approximation and molecular Ammosov-Delone-Krainov models. Our results demonstrate the feasibility of an all-optical approach for probing the ionization dynamics of lower-lying orbitals of molecules, which is until now still difficult to achieve by other techniques. Moreover, the deviation between the experimental and theoretical results indicates the incompleteness of current theoretical models for describing strong field ionization of molecules.; http://gateway.webofknowledge.com/gateway/Gateway.cgi?GWVersion=2&SrcApp=PARTNER_APP&SrcAuth=LinksAMR&KeyUT=WOS:000325364300009&DestLinkType=FullRecord&DestApp=ALL_WOS&UsrCustomerID=8e1609b174ce4e31116a60747a720701 ; Physics, Multidisciplinary; SCI(E); EI; 17; ARTICLE; 13; 111
语种英语
内容类型期刊论文
源URL[http://ir.pku.edu.cn/handle/20.500.11897/391096]  
专题工学院
推荐引用方式
GB/T 7714
Yao, Jinping,Li, Guihua,Jia, Xinyan,et al. Alignment-Dependent Fluorescence Emission Induced by Tunnel Ionization of Carbon Dioxide from Lower-Lying Orbitals[J]. 物理评论快报,2013.
APA Yao, Jinping.,Li, Guihua.,Jia, Xinyan.,Hao, Xiaolei.,Zeng, Bin.,...&Xu, Zhizhan.(2013).Alignment-Dependent Fluorescence Emission Induced by Tunnel Ionization of Carbon Dioxide from Lower-Lying Orbitals.物理评论快报.
MLA Yao, Jinping,et al."Alignment-Dependent Fluorescence Emission Induced by Tunnel Ionization of Carbon Dioxide from Lower-Lying Orbitals".物理评论快报 (2013).
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