Solid-State Water Electrolysis with an Alkaline Membrane | |
Leng, Yongjun ; Chen, Guang ; Mendoza, Alfonso J. ; Tighe, Timothy B. ; Hickner, Michael A. ; Wang, Chao-Yang | |
刊名 | journal of the american chemical society
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2012 | |
关键词 | ANION-EXCHANGE MEMBRANES HYDROGEN-PRODUCTION POLYMER ELECTROLYTE FUEL-CELLS PEM ELECTROLYSIS PERFORMANCE ENERGY ELECTROCATALYSIS STABILITY IONOMER |
DOI | 10.1021/ja302439z |
英文摘要 | We report high-performance, durable alkaline membrane water electrolysis in a solid-state cell. An anion exchange membrane (AEM) and catalyst layer ionomer for hydroxide ion conduction were used without the addition of liquid electrolyte. At 50 degrees C, an AEM electrolysis cell using iridium oxide as the anode catalyst and Pt black as the cathode catalyst exhibited a current density of 399 mA/cm(2) at 1.80 V. We found that the durability of the AEM-based electrolysis cell could be improved by incorporating a highly durable ionomer in the catalyst layer and optimizing the water feed configuration. We demonstrated an AEM-based electrolysis cell with a lifetime of > 535 h. These first-time results of water electrolysis in a solid-state membrane cell are promising for low-cost, scalable hydrogen production.; Chemistry, Multidisciplinary; SCI(E); EI; 0; ARTICLE; 22; 9054-9057; 134 |
语种 | 英语 |
内容类型 | 期刊论文 |
源URL | [http://ir.pku.edu.cn/handle/20.500.11897/233351] ![]() |
专题 | 工学院 |
推荐引用方式 GB/T 7714 | Leng, Yongjun,Chen, Guang,Mendoza, Alfonso J.,et al. Solid-State Water Electrolysis with an Alkaline Membrane[J]. journal of the american chemical society,2012. |
APA | Leng, Yongjun,Chen, Guang,Mendoza, Alfonso J.,Tighe, Timothy B.,Hickner, Michael A.,&Wang, Chao-Yang.(2012).Solid-State Water Electrolysis with an Alkaline Membrane.journal of the american chemical society. |
MLA | Leng, Yongjun,et al."Solid-State Water Electrolysis with an Alkaline Membrane".journal of the american chemical society (2012). |
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