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Spatial Distribution of Ozone Formation in China Derived from Emissions of Speciated Volatile Organic Compounds
Wu, Rongrong ; Xie, Shaodong
刊名ENVIRONMENTAL SCIENCE & TECHNOLOGY
2017
关键词PEARL RIVER DELTA INTERCOMPARISON PROJECT ACCMIP TROPOSPHERIC OZONE SURFACE OZONE ANTHROPOGENIC EMISSIONS ATMOSPHERIC CHEMISTRY SOURCE PROFILES AIR-QUALITY VOC SENSITIVITY
DOI10.1021/acs.est.6b03634
英文摘要Ozone (03) pollution is becoming increasingly severe in China. In addition, our limited understanding of the relationship between 03 and volatile organic compounds (VOCs), is an obstacle to improving air quality. By developing an improved source-oriented speciated VOC emission inventory in 2013, we estimated the ozone formation potential (OFP) and investigated its characteristics in China. Besides, a comparison was made between our estimates and space-based observations from the ozone monitoring instrument (OMI) on the National Aeronautics and Space Administration (NASA)'s Aura satellite. According to our estimates, m-/p-xylene, ethylene, formaldehyde, toluene, and propene were the five species that had the largest potential to form ozone, and on-road vehicles, industrial processes, biofuel combustion, and surface coating were the key contributing sectors. Among different regions of China, the North China Plain, Yangtze River Delta, and Pearl River Delta had the highest OFP values. Our results suggest that 03 formation is VOC-limited in major urban areas of China. Additionally, considering the different photochemical reactivities of various VOC species and the disparate energy and industry structures in the different regions of China, more efficient OFP-based and localized VOC control measures should be implemented, instead of the current mass-based and nationally uniform policies.; National Natural Science Foundation [91544106]; Environmental Protection Ministry of China [20130973]; SCI(E); ARTICLE; 5; 2574-2583; 51
语种英语
内容类型期刊论文
源URL[http://ir.pku.edu.cn/handle/20.500.11897/474649]  
专题环境科学与工程学院
推荐引用方式
GB/T 7714
Wu, Rongrong,Xie, Shaodong. Spatial Distribution of Ozone Formation in China Derived from Emissions of Speciated Volatile Organic Compounds[J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY,2017.
APA Wu, Rongrong,&Xie, Shaodong.(2017).Spatial Distribution of Ozone Formation in China Derived from Emissions of Speciated Volatile Organic Compounds.ENVIRONMENTAL SCIENCE & TECHNOLOGY.
MLA Wu, Rongrong,et al."Spatial Distribution of Ozone Formation in China Derived from Emissions of Speciated Volatile Organic Compounds".ENVIRONMENTAL SCIENCE & TECHNOLOGY (2017).
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