Temporal occurrence and sources of persistent organic pollutants in suspended particulate matter from the most heavily polluted river mouth of Lake Chaohu, China | |
Liu, Cheng ; Zhang, Lei ; Fan, Chengxin ; Xu, Fuliu ; Chen, Kaining ; Gu, Xiaozhi | |
刊名 | CHEMOSPHERE |
2017 | |
关键词 | Persistent organic pollutants Suspended particulate matter Potential risk Riverine Nanfei river Lake Chaohu POLYCYCLIC AROMATIC-HYDROCARBONS POLYBROMINATED DIPHENYL ETHERS ORGANOCHLORINE PESTICIDES OCPS COASTAL MARINE-SEDIMENTS SURFACE SEDIMENTS POLYCHLORINATED-BIPHENYLS TAIHU LAKE CONTAMINATED SEDIMENTS INCREASING LEVELS ECOLOGICAL RISKS |
DOI | 10.1016/j.chemosphere.2017.01.082 |
英文摘要 | The Nanfei River is by many measures the most heavily polluted tributary to Lake Chaohu. In this study, the temporal occurrence and sources of four classes of persistent organic pollutants (POPs), including polycyclic aromatic hydrocarbons (PAHs), organochlorine pesticides (OCPs), polybrominated diphenyl ethers (PBDEs), and polychlorinated biphenyls (PCBs), in suspended particulate matter (SPM) from the river mouth were investigated monthly during 2014. Results show that concentrations of all four POPs in SPM were higher than those in the sediment of Lake Chaohu. PBDEs (26.7 ng g(-1) dry weight (dw)) were originated mainly from commercial deca-BDE mixtures. PCB concentrations (1.336 ng dw) were lower than those of sediments in many other water bodies worldwide. PAHs (2597 ng g(-1) dw) and OCPs (5738 ng g(-1) dw) were the most common POPs. PAHs mainly had high molecular weights and originated from pyrolytic sources, with a small proportion of petrogenic origin. The predominant OCPs were DDT5, heptachlorep-oxides, dieldrin, hexachlorocyclohexanes, hexachlorobenzene, and chlordanes. Most OCPs originated from historical use, except lindane. Generally, of all the POPs studied, those of primary ecological concern should be acenaphthene, fluorene, DDT5, and chlordanes. Higher concentrations of POPs were detected during winter and spring than in summer and autumn, probably because of the high river flow during the rainy season. The high concentration of POPs in the riverine SPM and the fractionation of POPs in the water and SPM of the river should be a focal point in the future study of Lake Chaohu.(C) 2017 Elsevier Ltd. All rights reserved.; National Natural Science Foundation of China [41673123]; State Major Project for Water Pollution Control and Management [2012ZX07103-005, 2012ZX07103-002]; SCI(E); ARTICLE; 39-45; 174 |
语种 | 英语 |
内容类型 | 期刊论文 |
源URL | [http://ir.pku.edu.cn/handle/20.500.11897/473837] |
专题 | 城市与环境学院 |
推荐引用方式 GB/T 7714 | Liu, Cheng,Zhang, Lei,Fan, Chengxin,et al. Temporal occurrence and sources of persistent organic pollutants in suspended particulate matter from the most heavily polluted river mouth of Lake Chaohu, China[J]. CHEMOSPHERE,2017. |
APA | Liu, Cheng,Zhang, Lei,Fan, Chengxin,Xu, Fuliu,Chen, Kaining,&Gu, Xiaozhi.(2017).Temporal occurrence and sources of persistent organic pollutants in suspended particulate matter from the most heavily polluted river mouth of Lake Chaohu, China.CHEMOSPHERE. |
MLA | Liu, Cheng,et al."Temporal occurrence and sources of persistent organic pollutants in suspended particulate matter from the most heavily polluted river mouth of Lake Chaohu, China".CHEMOSPHERE (2017). |
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