Cumulative health risk assessment of halogenated and parent polycyclic aromatic hydrocarbons associated with particulate matters in urban air | |
Sun, Jian-Lin ; Jing, Xin ; Chang, Wen-Jing ; Chen, Zheng-Xia ; Zeng, Hui | |
刊名 | 生态毒物学与环境安全 |
2015 | |
关键词 | Halogenated polycyclic aromatic hydrocarbons Polycyclic aromatic hydrocarbons Particulate matter Health risk assessment Inhalation exposure LUNG-CANCER RISK HUMAN EXPOSURE SOUTH CHINA INHALATION EXPOSURE ELECTRONIC WASTE POLLUTION PAHS COMPLEX PM10 AREA |
DOI | 10.1016/j.ecoenv.2014.11.024 |
英文摘要 | Halogenated polycyclic aromatic hydrocarbons (HPAHs) have been reported to occur widely in urban air. Nevertheless, knowledge about the human health risk associated with inhalation exposure to HPAHs is scarce so far. In the present study, nine HPAHs and 16 PAHs were determined in atmospheric particulate matter (PM) collected from Shenzhen, China to address this issue. Concentrations of Sigma(9)HPAHs varied from 0.1 to 1.5 ng/m(3) and from 0.09 to 0.4 ng/m(3) in PM10 and PM2.5 samples, respectively. As for individuals, 9-bromoanthracene, 7-bromobenz(a)anthracene, and 9,10-dibromoanthracene were the dominant congeners. Levels of Sigma(16)PAHs in PM10 and PM2.5 samples ranged from 3.2 to 81 ng/m(3) and from 2.8 to 85 ng/m(3), respectively. Among individual PAHs, chrysene, benzo[b]fluoranthene, and indeno [1,2,3-c,d]pyrene were the main congeners. According to the season, concentrations of HPAHs and PAHs in atmospheric PM10/PM2.5 samples show a similar decreasing trend with an order: winter > autumn > spring > summer. The daily intake (DI) of PM10/PM2.5-bound HPAHs and PAHs were estimated. Our results indicated that children have the highest DI levels via inhalation exposure. The incremental lifetime cancer risk (ILCR) induced by PM10/PM2.5-bound HPAHs and PAHs were calculated. The ILCR values showed a similar decreasing trend with an order: adults > children > seniors > adolescent. Overall, the ILCR values induced by HPAHs and PAHs were far below the priority risk level (10(-4)), indicating no obvious cancer risk. To our knowledge, this is the first study to investigate the human health risk associated with inhalation exposure to PM10/PM2.5-bound HPAHs. (C) 2014 Elsevier Inc. All rights reserved.; http://gateway.webofknowledge.com/gateway/Gateway.cgi?GWVersion=2&SrcApp=PARTNER_APP&SrcAuth=LinksAMR&KeyUT=WOS:000348966400005&DestLinkType=FullRecord&DestApp=ALL_WOS&UsrCustomerID=8e1609b174ce4e31116a60747a720701 ; Environmental Sciences; Toxicology; SCI(E); PubMed; 5; ARTICLE; zenghui@pkusz.edu.cn; 31-37; 113 |
语种 | 英语 |
内容类型 | 期刊论文 |
源URL | [http://ir.pku.edu.cn/handle/20.500.11897/160530] |
专题 | 城市与环境学院 |
推荐引用方式 GB/T 7714 | Sun, Jian-Lin,Jing, Xin,Chang, Wen-Jing,et al. Cumulative health risk assessment of halogenated and parent polycyclic aromatic hydrocarbons associated with particulate matters in urban air[J]. 生态毒物学与环境安全,2015. |
APA | Sun, Jian-Lin,Jing, Xin,Chang, Wen-Jing,Chen, Zheng-Xia,&Zeng, Hui.(2015).Cumulative health risk assessment of halogenated and parent polycyclic aromatic hydrocarbons associated with particulate matters in urban air.生态毒物学与环境安全. |
MLA | Sun, Jian-Lin,et al."Cumulative health risk assessment of halogenated and parent polycyclic aromatic hydrocarbons associated with particulate matters in urban air".生态毒物学与环境安全 (2015). |
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