Gray Ta2O5 Nanowires with Greatly Enhanced Photocatalytic Performance | |
Zhu, Guilian ; Lin, Tianquan ; Cui, Houlei ; Zhao, Wenli ; Zhang, Hui ; Huang, Fuqiang | |
刊名 | ACS APPLIED MATERIALS & INTERFACES |
2016 | |
关键词 | Ta2O5 nanowire aluminum reduction photocatalysis PEC SOLAR-ENERGY UTILIZATION TIO2 NANOTUBE ARRAYS VISIBLE-LIGHT THIN-FILMS HYDROGEN-PRODUCTION THERMAL-TREATMENT TANTALUM OXIDE NANOPARTICLES ABSORPTION OXIDATION |
DOI | 10.1021/acsami.5b07685 |
英文摘要 | Black TiO2, with enhanced solar absorption and photocatalytic activity, has gained extensive attention, inspiring us to investigate the reduction of other wide-bandgap semiconductors for improved performance. Herein, we report the preparation of gray Ta2O5 nanowires with disordered shells and abundant defects via aluminum reduction. Its water decontamination is 2.5 times faster and hydrogen production is 2.3-fold higher over pristine Ta2O5. The reduced Ta2O5 also delivers significantly enhanced photoelectrochemical performance compared with the pristine Ta2O5 nanowires, including much higher carrier concentration, easier electron-hole separation and 11 times larger photocurrent. Our results demonstrate that Ta2O5 will have great potentials in photocatalysis and solar energy utilization after proper modification.; National Natural Science Foundation of China; Science and Technology Commission of Shanghai; SCI(E); EI; ARTICLE; zhanghui@mail.sic.ac.cn; huangfq@mail.sic.ac.cn; 1; 122-127; 8 |
语种 | 英语 |
内容类型 | 期刊论文 |
源URL | [http://ir.pku.edu.cn/handle/20.500.11897/437825] |
专题 | 化学与分子工程学院 |
推荐引用方式 GB/T 7714 | Zhu, Guilian,Lin, Tianquan,Cui, Houlei,et al. Gray Ta2O5 Nanowires with Greatly Enhanced Photocatalytic Performance[J]. ACS APPLIED MATERIALS & INTERFACES,2016. |
APA | Zhu, Guilian,Lin, Tianquan,Cui, Houlei,Zhao, Wenli,Zhang, Hui,&Huang, Fuqiang.(2016).Gray Ta2O5 Nanowires with Greatly Enhanced Photocatalytic Performance.ACS APPLIED MATERIALS & INTERFACES. |
MLA | Zhu, Guilian,et al."Gray Ta2O5 Nanowires with Greatly Enhanced Photocatalytic Performance".ACS APPLIED MATERIALS & INTERFACES (2016). |
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