Toward Single-Layer Uniform Hexagonal Boron Nitride-Graphene Patchworks with Zigzag Linking Edges | |
Gao, Yabo ; Zhang, Yanfeng ; Chen, Pengcheng ; Li, Yuanchang ; Liu, Mengxi ; Gao, Teng ; Ma, Donglin ; Chen, Yubin ; Cheng, Zhihai ; Qju, Xiaohui ; Duan, Wenhui ; Liu, Zhongfan | |
刊名 | nano letters |
2013 | |
关键词 | graphene boron nitride BNC hybrid interface STM NANOMESH HETEROSTRUCTURES NANORIBBONS MONOLAYER NANOTUBES BANDGAP HALF GAP |
DOI | 10.1021/nl4021123 |
英文摘要 | The atomic layer of hybridized, hexagonal boron nitride (h-BN) and graphene has attracted a great deal of attention after the pioneering work of P. M. Ajayan et al. on Cu foils because of their unusual electronic properties (Ci, L. J.; et al. Nat. Mater. 2010, 9, 430-435). However, many fundamental issues are still not clear, including the in-plane atomic continuity as well as the edge type at the boundary of hybridized h-BN and graphene domains. To clarify these issues, we have successfully grown a perfect single-layer h-BN-graphene (BNC) patchwork on a selected Rh(111) substrate, via a two-step patching growth approach. With the ideal sample, we convinced that at the in-plane linking interface, graphene and h-BN can be linked perfectly at an atomic scale. More importantly, we found that zigzag linking edges were preferably formed, as demonstrated by atomic-scale scanning tunneling microscopy images, Which was also theoretically verified using density functional theory calculations. We believe the experimental and theoretical works are of particular importance to obtain a fundamental understanding of the BNC hybrid and to establish a deliberate structural, control targeting high-performance electronic and spintronic devices.; Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter; SCI(E); EI; PubMed; 34; ARTICLE; 7; 3439-3443; 13 |
语种 | 英语 |
内容类型 | 期刊论文 |
源URL | [http://ir.pku.edu.cn/handle/20.500.11897/149752] |
专题 | 化学与分子工程学院 工学院 |
推荐引用方式 GB/T 7714 | Gao, Yabo,Zhang, Yanfeng,Chen, Pengcheng,et al. Toward Single-Layer Uniform Hexagonal Boron Nitride-Graphene Patchworks with Zigzag Linking Edges[J]. nano letters,2013. |
APA | Gao, Yabo.,Zhang, Yanfeng.,Chen, Pengcheng.,Li, Yuanchang.,Liu, Mengxi.,...&Liu, Zhongfan.(2013).Toward Single-Layer Uniform Hexagonal Boron Nitride-Graphene Patchworks with Zigzag Linking Edges.nano letters. |
MLA | Gao, Yabo,et al."Toward Single-Layer Uniform Hexagonal Boron Nitride-Graphene Patchworks with Zigzag Linking Edges".nano letters (2013). |
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