Crude oil removal from aqueous solution using raw and carbonized Xanthoceras sorbifolia shells
Liu, Linan3,4; Wang, Lihua3; Song, Wenhong3; Yang, Liang1; Yin, Liming3; Xia, Shaopan4; Wang, Hailong2,5; Strong, Peter James6; Song, Zhaoliang4
刊名ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH
2018-10-01
卷号25期号:29页码:29325-29334
关键词Adsorption kinetics Biosorbents Oily wastewater Physical-chemistry adsorption Saponin
ISSN号0944-1344
DOI10.1007/s11356-018-2895-0
英文摘要Fruit shell residue from Xanthoceras sorbifolia was investigated as a potential biosorbent to remove crude oil from aqueous solution. The shell powder and its carbonized material were compared while assessing various factors that influenced oil removal capacity. The structure and sorption mechanism were characterized using scanning electron microscopy and Fourier-transform infrared spectroscopy. The oil removal capacity of the raw material (75.1 mg g(-1)) was better than the carbonized material (49.5 mg g(-1)). The oil removal capacity increased with greater saponin content, indicating that hydrophobic and lipophilic surface characteristics of the saponins improved adsorption by the raw X. sorbifolia shell. An orthogonal experimental design was used to optimize the adsorption. Using 4gL(-1) of raw X. sorbifolia shell (particle size of < 0.15 mm), the highest crude oil removal efficiency was obtained using an initial oil concentration of 400 mg L-1, adsorption temperature of 30 degrees C, adsorption time of 10 min at a shaking speed of 150 rpm. The adsorption of crude oil onto X. sorbifolia shell was best described using a pseudo-second-order kinetic model. Raw X. sorbifolia shell material was more efficient than the carbonized material at crude oil removal from aqueous solution. This was attributable to the functional groups of saponins in raw X. sorbifolia shell. This study highlights that some agricultural and forest residues could be a promising source of low-cost biosorbents for oil contaminants from water-without requiring additional processing such as carbonization.
资助项目National "Twelfth Five-Year" Plan for Science & Technology Support of China[2012BAD32B08] ; Natural Science Foundation of Guangdong Province, China[2017A030311019]
WOS研究方向Environmental Sciences & Ecology
语种英语
出版者SPRINGER HEIDELBERG
WOS记录号WOS:000445273500053
内容类型期刊论文
源URL[http://210.72.129.5/handle/321005/123230]  
专题中国科学院沈阳应用生态研究所
通讯作者Wang, Lihua; Song, Zhaoliang
作者单位1.Shenyang Agr Univ, Coll Land & Environm, Shenyang 110866, Liaoning, Peoples R China
2.Foshan Univ, Sch Environm & Chem Engn, Foshan 528000, Guangdong, Peoples R China
3.Chinese Acad Sci, Inst Appl Ecol, Shenyang 110016, Liaoning, Peoples R China
4.Tianjin Univ, Inst Surface Earth Syst Sci, Tianjin 300072, Peoples R China
5.Zhejiang A&F Univ, Sch Environm & Resource Sci, Hangzhou 311300, Zhejiang, Peoples R China
6.Queensland Univ Technol, GPO Box 2432,2 George St, Brisbane, Qld 4001, Australia
推荐引用方式
GB/T 7714
Liu, Linan,Wang, Lihua,Song, Wenhong,et al. Crude oil removal from aqueous solution using raw and carbonized Xanthoceras sorbifolia shells[J]. ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH,2018,25(29):29325-29334.
APA Liu, Linan.,Wang, Lihua.,Song, Wenhong.,Yang, Liang.,Yin, Liming.,...&Song, Zhaoliang.(2018).Crude oil removal from aqueous solution using raw and carbonized Xanthoceras sorbifolia shells.ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH,25(29),29325-29334.
MLA Liu, Linan,et al."Crude oil removal from aqueous solution using raw and carbonized Xanthoceras sorbifolia shells".ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH 25.29(2018):29325-29334.
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