CeO2-WO3 Mixed Oxides for the Selective Catalytic Reduction of NOx by NH3 Over a Wide Temperature Range | |
Chen, Liang1,2,3; Li, Junhua1,4; Ablikim, Wijdan1; Wang, Jun1; Chang, Huazhen1; Ma, Lei1; Xu, Jiayu1; Ge, Maofa3; Arandiyan, Hamidreza1 | |
刊名 | CATALYSIS LETTERS |
2011-12-01 | |
卷号 | 141期号:12页码:1859-1864 |
关键词 | Nox Scr Ceo2-wo3 Interaction Lattice Nh3 So2 |
ISSN号 | 1011-372X |
DOI | 10.1007/s10562-011-0701-4 |
英文摘要 | A series of cerium-tungsten oxide catalysts was prepared by the co-precipitation method and was evaluated for the selective catalytic reduction of NOx by ammonia (NH3-SCR) over a wide temperature range. These catalysts were characterized by BET, XRD, XPS and H-2-TPR analyses. The experimental studies demonstrated that, among cerium-tungsten oxides, CeO2-WO3 with a Ce/W molar ratio of 3/2 exhibited the best activity toward NH3SCR reactions, N-2 selectivity and SO2 durability over a broad temperature range of 175-500 degrees C at a space velocity of 47,000 h(-1). The strong interaction between Ce and W could be the main factor leading to the high activity of the CeO2-WO3 mixed oxide catalyst. |
语种 | 英语 |
出版者 | SPRINGER |
WOS记录号 | WOS:000299919300018 |
内容类型 | 期刊论文 |
源URL | [http://ir.iccas.ac.cn/handle/121111/71363] |
专题 | 中国科学院化学研究所 |
通讯作者 | Li, Junhua |
作者单位 | 1.Tsinghua Univ, Sch Environm, Beijing 100084, Peoples R China 2.CPI Yuanda Envirom Protect Engn Co Ltd, Chongqing, Peoples R China 3.Chinese Acad Sci, Inst Chem, Beijing Natl Lab Mol Sci BNLMS, Beijing 100190, Peoples R China 4.Tsinghua Univ, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100084, Peoples R China |
推荐引用方式 GB/T 7714 | Chen, Liang,Li, Junhua,Ablikim, Wijdan,et al. CeO2-WO3 Mixed Oxides for the Selective Catalytic Reduction of NOx by NH3 Over a Wide Temperature Range[J]. CATALYSIS LETTERS,2011,141(12):1859-1864. |
APA | Chen, Liang.,Li, Junhua.,Ablikim, Wijdan.,Wang, Jun.,Chang, Huazhen.,...&Arandiyan, Hamidreza.(2011).CeO2-WO3 Mixed Oxides for the Selective Catalytic Reduction of NOx by NH3 Over a Wide Temperature Range.CATALYSIS LETTERS,141(12),1859-1864. |
MLA | Chen, Liang,et al."CeO2-WO3 Mixed Oxides for the Selective Catalytic Reduction of NOx by NH3 Over a Wide Temperature Range".CATALYSIS LETTERS 141.12(2011):1859-1864. |
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