A robust fuel cell cathode catalyst assembled with nitrogen-doped carbon nanohorn and platinum nanoclusters | |
Zhang, Linwei1,2; Zheng, Ning1; Gao, Ang1; Zhu, Chunmei1; Wang, Zhiyong1; Wang, Yuan1; Shi, Zujin1; Liu, Yan1 | |
刊名 | JOURNAL OF POWER SOURCES
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2012-12-15 | |
卷号 | 220页码:449-454 |
关键词 | Catalytic Cathode Durability Nitrogen-doped Oxygen Reduction Reaction Polymer Electrolyte Membrane Fuel Cells |
ISSN号 | 0378-7753 |
DOI | 10.1016/j.jpowsour.2012.08.009 |
英文摘要 | A highly durable and active nanocomposite cathode catalyst (Pt/NSWCNH) is assembled with "unprotected" Pt nanoclusters and nitrogen-doped single-wall carbon nanohorns (NSWCNH) as building blocks by a convenient process. The specific catalytic activity and mass catalytic activity for the oxygen reduction reaction over Pt/NSWCNH is 1.60 and 1.75 times as high as those over a commercial Pt/C catalyst, respectively. There is no obvious loss in the catalytic activity of Pt/NSWCNH after potential cycling from 0.6 to 1.1 V versus RHE for 15,000 cycles at 30 degrees C, under the oxidizing conditions for the electrochemically catalytic reduction of O-2. TEM characterization results reveal that, during the accelerated aging tests, Pt nanoparticles in Pt/NSWCNH are more stable than that in Pt/C-JM, showing a low increase in the particle size. (C) 2012 Elsevier B.V. All rights reserved. |
语种 | 英语 |
出版者 | ELSEVIER SCIENCE BV |
WOS记录号 | WOS:000309990300060 |
内容类型 | 期刊论文 |
源URL | [http://ir.iccas.ac.cn/handle/121111/48897] ![]() |
专题 | 中国科学院化学研究所 |
通讯作者 | Wang, Yuan |
作者单位 | 1.Peking Univ, Beijing Natl Lab Mol Sci, Coll Chem & Mol Engn, State Key Lab Struct Chem Unstable & Stable Speci, Beijing 100871, Peoples R China 2.Lanzhou Univ, Coll Chem & Chem Engn, Lanzhou 730000, Peoples R China |
推荐引用方式 GB/T 7714 | Zhang, Linwei,Zheng, Ning,Gao, Ang,et al. A robust fuel cell cathode catalyst assembled with nitrogen-doped carbon nanohorn and platinum nanoclusters[J]. JOURNAL OF POWER SOURCES,2012,220:449-454. |
APA | Zhang, Linwei.,Zheng, Ning.,Gao, Ang.,Zhu, Chunmei.,Wang, Zhiyong.,...&Liu, Yan.(2012).A robust fuel cell cathode catalyst assembled with nitrogen-doped carbon nanohorn and platinum nanoclusters.JOURNAL OF POWER SOURCES,220,449-454. |
MLA | Zhang, Linwei,et al."A robust fuel cell cathode catalyst assembled with nitrogen-doped carbon nanohorn and platinum nanoclusters".JOURNAL OF POWER SOURCES 220(2012):449-454. |
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