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Constructing a Stable Lithium Metal-Gel Electrolyte Interface for Quasi-Solid-State Lithium Batteries
Zuo, Tong-Tong1,3; Shi, Yang1,3; Wu, Xiong-Wei2; Wang, Peng-Fei1,3; Wang, Shu-Hua1; Yin, Ya-Xia1,3; Wang, Wen-Peng1,3; Ma, Qiang1,2; Zeng, Xian-Xiang1,2; Ye, Huan1
刊名ACS APPLIED MATERIALS & INTERFACES
2018-09-12
卷号10期号:36页码:30065-30070
关键词Li Metal Batteries Li Metal Anode Gel Electrolyte Interfacial Stability Solid-state Batteries Double Polymer Network
ISSN号1944-8244
DOI10.1021/acsami.8b12986
英文摘要Interfacial problems, including interfacial stability and contact issues, severely plague the practical application of Li metal anodes. Here we report an interfacial regulation strategy that stabilizes the Li metal-gel electrolyte interface through in situ constructing a stable solid electrolyte interphase (SEI) layer. By stabilizing the interface of Li metal anodes, the gel electrolyte enables dendrite-free morphology and high plating/stripping efficiency. A systematic analysis further confirms that the formed SEI layer is responsible for homogeneous deposition and stable cycling performance. Benefiting from the interfacial stability between electrodes and electrolytes, the lifespan of Li metal batteries is extended.
语种英语
出版者AMER CHEMICAL SOC
WOS记录号WOS:000444793000009
内容类型期刊论文
源URL[http://ir.iccas.ac.cn/handle/121111/43055]  
专题中国科学院化学研究所
通讯作者Wen, Rui; Guo, Yu-Guo
作者单位1.Chinese Acad Sci, Inst Chem, CAS Res Educ Ctr Excellence Mol Sci, CAS Key Lab Mol Nanostruct & Nanotechnol, Beijing 100190, Peoples R China
2.Hunan Agr Univ, Coll Sci, Changsha 410128, Hunan, Peoples R China
3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
推荐引用方式
GB/T 7714
Zuo, Tong-Tong,Shi, Yang,Wu, Xiong-Wei,et al. Constructing a Stable Lithium Metal-Gel Electrolyte Interface for Quasi-Solid-State Lithium Batteries[J]. ACS APPLIED MATERIALS & INTERFACES,2018,10(36):30065-30070.
APA Zuo, Tong-Tong.,Shi, Yang.,Wu, Xiong-Wei.,Wang, Peng-Fei.,Wang, Shu-Hua.,...&Guo, Yu-Guo.(2018).Constructing a Stable Lithium Metal-Gel Electrolyte Interface for Quasi-Solid-State Lithium Batteries.ACS APPLIED MATERIALS & INTERFACES,10(36),30065-30070.
MLA Zuo, Tong-Tong,et al."Constructing a Stable Lithium Metal-Gel Electrolyte Interface for Quasi-Solid-State Lithium Batteries".ACS APPLIED MATERIALS & INTERFACES 10.36(2018):30065-30070.
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