A general printing approach for scalable growth of perovskite single-crystal films | |
Gu, Zhenkun1,2; Huang, Zhandong1,2; Li, Chang1,2; Li, Mingzhu1; Song, Yanlin1 | |
刊名 | SCIENCE ADVANCES |
2018-06-01 | |
卷号 | 4期号:6 |
ISSN号 | 2375-2548 |
DOI | 10.1126/sciadv.aat2390 |
英文摘要 | Perovskite single-crystal films, which exhibit exceptionally low trap density and nearly perfect translational symmetry, are believed to achieve the highest performance of perovskite-based optoelectronic devices. However, fabrication of these perovskite single-crystal films is quite difficult because of the uncontrollable nucleation caused by the rapid reaction of two perovskite precursors. We report a facile seed printing approach to selectively create millimeter-sized perovskite single-crystal films with controlled thickness and high yield. We show that perovskite single-crystal films can be perfectly transferred to almost arbitrary substrates through the printing process. The as-grown perovskite single-crystal films have excellent crystalline quality and morphology. We further demonstrate that perovskite single-crystal films can be directly printed for scalable fabrication of photodetectors and effective image sensors. This strategy allows high-yield fabrication of large perovskite single-crystal films for functional devices and may extend to other solution-processed materials for wide applications. |
语种 | 英语 |
出版者 | AMER ASSOC ADVANCEMENT SCIENCE |
WOS记录号 | WOS:000443175500074 |
内容类型 | 期刊论文 |
源URL | [http://ir.iccas.ac.cn/handle/121111/42327] |
专题 | 中国科学院化学研究所 |
通讯作者 | Li, Mingzhu; Song, Yanlin |
作者单位 | 1.Chinese Acad Sci, Beijing Engn Res Ctr Nanomat Green Printing Techn, Beijing Natl Lab Mol Sci, Key Lab Green Printing,Inst Chem, Beijing 100190, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
推荐引用方式 GB/T 7714 | Gu, Zhenkun,Huang, Zhandong,Li, Chang,et al. A general printing approach for scalable growth of perovskite single-crystal films[J]. SCIENCE ADVANCES,2018,4(6). |
APA | Gu, Zhenkun,Huang, Zhandong,Li, Chang,Li, Mingzhu,&Song, Yanlin.(2018).A general printing approach for scalable growth of perovskite single-crystal films.SCIENCE ADVANCES,4(6). |
MLA | Gu, Zhenkun,et al."A general printing approach for scalable growth of perovskite single-crystal films".SCIENCE ADVANCES 4.6(2018). |
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