Multimedia fate and transport simulation of perfluorooctanoic acid/perfluorooctanoate in an urbanizing area | |
Meng, Jing; Lu, Xiaotian; Su, Chao; Song, Shuai; Lu, Yonglong; Wang, Pei; Juergens, Monika D.; Khan, Kifayatullah; Baninla, Yvette; Liang, Ruoyu | |
刊名 | SCIENCE OF THE TOTAL ENVIRONMENT |
2018-12-01 | |
卷号 | 643页码:90-97 |
关键词 | PFOA/PFO Multimedia model Hydrosphere Coastal region China |
ISSN号 | 0048-9697 |
文献子类 | Article |
英文摘要 | Strong global demand leads to significant production of fluoropolymers (FP) in China which potentially release large quantities of perfluorooctanoic acid/perfluorooctanoate (collectively called PFOA/PFO) to the environment. Modelling the fate and transport of PFOA/PFO provides an important input for human health risk assessment. Considering the effects of urbanization and existing forms of PFOA/PFO, this study used the modified multispecies Berkeley-Trent-Urban-Rural model to simulate the transfer behavior of PFOA/PFO in the Bohai Rim, China. Spatial distributions of PFOA/PFO emissions during the year 2012 for the study area were illustrated. About two thirds of the total amount of PFOA/PFO was estimated to be released into fresh water, and the total releases to rural areas were 160-fold higher than those to urban areas due to the location of fluorochemical industrial parks. The simulations predicted that hydrosphere was the fate of PFOA/PFO, followed by soil and vegetation, which was consistent with field data. The highest PFOA/PFO concentration was modeled in the Xiaoqing River basin with a value of 32.57 mu g/L. The PFOA/PFO concentrations in urban soils were generally higher than those in rural soils except for grids 1, 3 and 46. In addition, it was estimated that the total flux of PFOA/PFO entering into the Bohai Sea was 24.57 ton/year, 100-fold higher than that of perfluorooctane sulfonates (PFOS). (C) 2018 Elsevier B.V. All rights reserved. |
内容类型 | 期刊论文 |
源URL | [http://ir.rcees.ac.cn/handle/311016/40613] |
专题 | 生态环境研究中心_城市与区域生态国家重点实验室 |
推荐引用方式 GB/T 7714 | Meng, Jing,Lu, Xiaotian,Su, Chao,et al. Multimedia fate and transport simulation of perfluorooctanoic acid/perfluorooctanoate in an urbanizing area[J]. SCIENCE OF THE TOTAL ENVIRONMENT,2018,643:90-97. |
APA | Meng, Jing.,Lu, Xiaotian.,Su, Chao.,Song, Shuai.,Lu, Yonglong.,...&Liang, Ruoyu.(2018).Multimedia fate and transport simulation of perfluorooctanoic acid/perfluorooctanoate in an urbanizing area.SCIENCE OF THE TOTAL ENVIRONMENT,643,90-97. |
MLA | Meng, Jing,et al."Multimedia fate and transport simulation of perfluorooctanoic acid/perfluorooctanoate in an urbanizing area".SCIENCE OF THE TOTAL ENVIRONMENT 643(2018):90-97. |
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