Geochemical valuation and intake of F, As, and Se in coal wastes contaminated areas and their potential impacts on local inhabitants, Shaanxi China

doi:10.1007/s10653-018-0131-y

	Geochemical valuation and intake of F, As, and Se in coal wastes contaminated areas and their potential impacts on local inhabitants, Shaanxi China
	Hussain, Rahib 1,2; Luo, Kunli 1
刊名	ENVIRONMENTAL GEOCHEMISTRY AND HEALTH
	2018-12-01
卷号	40 期号:6 页码:2667-2683
关键词	Cambrian Fluoride Jurassic Selenium Toxicity Weibei coalfield
ISSN号	0269-4042
DOI	10.1007/s10653-018-0131-y
通讯作者	Luo, Kunli(luokl@igsnrr.ac.cn)
英文摘要	This study probe the human health risk of fluoride (F), arsenic (As), and selenium (Se) and their daily intake available quantity to human through different sources in different regions of Shaanxi, China. For this purpose, a number of samples, including coal and coal wastes, rocks, soil, and vegetables were collected from south Qinling Mountain stone-like coal (Geo type-I), Binxian-Jurassic (Geo type-II), Hancheng Permo-Carboniferous (Geo type-III), and countryside (Huanglong County) of Shaanxi province. All these samples were analyzed through atomic fluorescence spectroscopy and combustion hydrolysis methods. Results showed that Geo type-I was enriched with As, Se, and F, Geo type-II, III, and the countryside were slightly enriched with As and F and deficient in Se. The average daily intake (ADI) of Se in Geo type-I was 0.005-0.0045, Geo type-II 0.0005-0.0004, Geo type-III 0.0006-0.0005, and countryside 0.0002-0.001 in mg kg(-1) day(-1) adult-children, respectively, which was lower than the optimum level (0.06-0.075 mg kg(-1) day(-1)). ADI of As at Geo type-I was 0.0085-0.0075, Geo type-II 0.004-0.0037, Geo type-III 0.0008, and countryside 0.00022-0.00019 in mg kg(-1)day(-1) adult-children, respectively, which was above the acceptable range (10(-6)-10(-4)). ADI of F at Geo type-I was 0.0047-0.0041, Geo type-II 0.0098-0.0087, Geo type-III 0.002-0.0017 and countryside 0.0015-0.0013 in mg kg(-1) day(-1) adult-children, respectively. The toxicity level of Se and F at all the regions was lower than the NOAEL and LOAEL, while As was higher at Geo type-II and I. The extreme deficient of Se than the optimum range along with high F could deregulatethe normal body growth especially causes bones and joint problems. However, the study found a rare patient with bone and joint disease (maybe Kashin-Beck disease) in the countryside. To find the exact cause of Kashin-Beck disease, the study needs further medical investigation in Se-deficient regions and their association with selenium deficiency and enriched fluoride.
资助项目	National Basic Research Program of China[2014CB238906] ; National Basic Research Program of China[AA17202026] ; National Natural Science Foundation of China[41172310] ; National Natural Science Foundation of China[41472322] ; CAS-TWAS Ph.D. fellowship
WOS关键词	ROASTED CORN ; SELENIUM ; FLUORINE ; FLUOROSIS ; EMISSION ; SOIL ; COMBUSTION ; COALFIELD ; CHILDREN ; PROVINCE
WOS研究方向	Engineering ; Environmental Sciences & Ecology ; Public, Environmental & Occupational Health ; Water Resources
语种	英语
出版者	SPRINGER
WOS记录号	WOS:000452307100026
资助机构	National Basic Research Program of China ; National Natural Science Foundation of China ; CAS-TWAS Ph.D. fellowship
内容类型	期刊论文
源URL	[http://ir.igsnrr.ac.cn/handle/311030/51315]
专题	中国科学院地理科学与资源研究所
通讯作者	Luo, Kunli
作者单位	1.Inst Geog Sci & Nat Resource Res, Beijing 100101, Peoples R China 2.Univ Chinese Acad Sci, Beijing 10080, Peoples R China
推荐引用方式 GB/T 7714	Hussain, Rahib,Luo, Kunli. Geochemical valuation and intake of F, As, and Se in coal wastes contaminated areas and their potential impacts on local inhabitants, Shaanxi China[J]. ENVIRONMENTAL GEOCHEMISTRY AND HEALTH,2018,40(6):2667-2683.
APA	Hussain, Rahib,&Luo, Kunli.(2018).Geochemical valuation and intake of F, As, and Se in coal wastes contaminated areas and their potential impacts on local inhabitants, Shaanxi China.ENVIRONMENTAL GEOCHEMISTRY AND HEALTH,40(6),2667-2683.
MLA	Hussain, Rahib,et al."Geochemical valuation and intake of F, As, and Se in coal wastes contaminated areas and their potential impacts on local inhabitants, Shaanxi China".ENVIRONMENTAL GEOCHEMISTRY AND HEALTH 40.6(2018):2667-2683.